Developing approaches for precise engineering of the optical response of plasmonic nanocavities at the post-fabrication stage is important for achieving enhanced and tunable light-matter interactions. In this work, we demonstrate selective enhancement/suppression of specific plasmonic modes by embedding nanocube-on-mirror plasmonic nanocavities into a poly(methyl methacrylate) (PMMA) layer with a controllable thickness. With the increase of the PMMA thickness from 0 to approximately 100 nm, the dominating out-of-plane plasmonic modes are significantly suppressed in the scattering spectra, while the in-plane plasmonic modes are greatly enhanced with a factor reaching 102±20. This enhancement is related to the variation of momentum matching between the plasmonic modes and the radiative fields, affecting both mode excitation and emission properties. In addition, the spectral positions of the in-plane and out-of-plane plasmonic modes shift up to 52±5 and 81±2 nm, respectively. These properties are important for matching and enhancing plasmonic and molecular resonances in a variety of applications.

The high degree of freedom of multimechanism metasurfaces has greatly facilitated multifunction or even multiphysics design for practical applications. In this work, to achieve camouflages simultaneously in microwave, infrared, and optical regimes, we propose a multimechanism-empowered metasurface composed of four elemental indium-tin-oxide-based meta-atoms. Each meta-atom can modulate microwaves both in phase and magnitude through polarization conversion and resonance absorption, which can realize radar stealth at 8–14 GHz. The reflective amplitude is less than -10 dB. When the incident angle increases to 60°, the reflective amplitude is still less than -3 dB. The far-field scattering patterns of microwaves are modulated by destructive interferences of reflected waves, which results in diffusion-like scattering due to randomly distributed reflection phases on the metasurface. The superposition of microwave absorption and diffuse reflection enables broadband microwave scattering reduction of the metasurface. Meanwhile, the emissivity of four types of meta-atoms covers from 0.3–0.8 at 3–14 μm due to delicately designed occupation ratios. The infrared radiation of the metasurface exhibits the characteristics of digital camouflage in infrared imaging. To demonstrate this method, prototypes were fabricated and measured. The measured results are consistent with the simulated ones. The angular stability in the microwave range within 0°–60° was also demonstrated. This work presents an approach to achieving multispectrum functions with integrated multimechanisms in a single functional metasurface layer and offers a new methodology for custom-designing infrared performance. Moreover, the simplicity of the structure offers significant cost control and large-scale fabrication advantages.

In this paper, a method to excite chiral quasi-bound states in the continuum (Q-BICs) using an asymmetric interface is proposed for the first time, to our knowledge. The chirality of a metasurface can be controlled by varying the medium of the active layer, achieving a maximum circular dichroism (CD) value of 0.9. Two types of reconfigurable chiral Q-BIC metasurfaces, a single-biased chiral Q-BIC metasurface (SBCBM) and a dual-biased chiral Q-BIC metasurface (DBCBM), are proposed, facilitated by the use of the electronically controlled material polyaniline (PANI). This enables electrically reconfigurable chiral Q-BIC with a maximum CD variability range from -0.9 to +0.9. These results highlight significant potential applications in fields such as reconfigurable devices, optical chiral switching, and environmental monitoring.

Manipulating hyperbolic polaritons at infrared frequencies has recently garnered interest as it promises to deliver new functionality for next-generation optical and photonic devices. This study investigates the impact of the crystal’s anisotropy orientation on the attenuated total reflection (ATR) spectra, more specifically, revealing the optical footprint of elliptical, ghost (GHP), and leaky (LHP) hyperbolic polaritons. Our findings reveal that the ATR spectra of GHPs exhibit a distinct hyperbolic behavior that is similar to that recently observed using s-SNOM techniques. Similarly, the ATR spectra of LHPs show its clear lenticular behavior; however, here we are able to discern the effects of large asymmetry due to cross polarization conversion when the crystal anisotropy is tilted away from the surface. Furthermore, we demonstrate that by controlling the anisotropy orientation of hyperbolic media it is possible to significantly alter the optical response of these polaritons. Thus, our results provide a foundation for the design of direction-dependent optical devices.

Traditional tunable metasurfaces have evolved through mechanisms relying on external stimuli, such as electrical, thermal, or optical excitation, to dynamically control electromagnetic (EM) wavefronts. While these approaches enable functionalities like focal varying and polarization modulation, they suffer from inherent limitations, including energy inefficiency, structural complexity, and limited adaptability. Here, cascaded all-dielectric Moiré metasurfaces are introduced, which are capable of simultaneous polarization multiplexing and focal-length control for terahertz (THz) beams without external stimuli. Moiré device 1 combines polarization-insensitive (Layer 1) and polarization-sensitive (Layer 2) meta-atoms to independently tailor orthogonal circular polarization channels, including left-handed circular polarization (LCP) and right-handed circular polarization (RCP). Under circularly polarized illumination, it generates focused beams with distinct topological charges (l=0 for LCP→RCP and l=1 for RCP→LCP), while relative layer rotation enables continuous focal-length adjustment from 9.28 mm to 3.22 mm, accompanied by a numerical aperture (NA) increase from 0.54 to 0.88. Moiré device 2 extends this paradigm to orthogonal linear polarization (LP) channels, producing l=1 and l=0 beams under x-LP and y-LP illumination, with a zoom range of 8.42–3.11 mm and NA up to 0.88. Experimental results validate polarization-selective focusing with efficiency exceeding 15% and robust agreement with simulation results, and the calculated absolute percentage errors (APEs) are below 5.9% for focal length and 3% for NA. These values are consistent with the expected theoretical trends, demonstrating that the experimental results align well with the predicted performance. This reconfigurable system introduces additional control dimensions through mechanical adjustments to cascaded metasurfaces, paving the way for adaptive wavefront control and opening new avenues for next-generation optical technologies.

Surface plasmonic polaritons (SPPs) break Abbe’s diffraction limit in the near field and provide a promising solution for high-resolution nanolithography without reducing illuminating wavelength. However, the resolution of the normal plasmonic lithography method based on ultraviolet exposure of a photoresist heavily relies on the size of the elaborate nanostructures, which usually require precise nanofabrication. Meanwhile, a high-cost pulsed laser is required as the light source to further reduce the lithography linewidth. Here, we establish a high-resolution and low-cost scanning probe nanolithography system based on the infrared surface plasmons. An easy-fabrication probe is designed by tailoring four concentric annular slits with a moderate width of 200 nm, which couples the incident radially polarized beam into SPPs, resulting in an ultra-strong spot at the tip apex. Such superfocusing mode is demonstrated to apply to the thermal field through the optical-thermal effect so as to cause the heat accumulation with a more restricted heating area, which is utilized for the thermal probe nanolithography. Experimental results indicate that the subwavelength feature with a linewidth down to 13 nm is realized using an inexpensive 1064 nm wavelength continuous-wave laser. Our scheme shows great potential in fabrication of planar optical elements with small size and high flexibility, and can also find extensive applications in areas such as single-molecule spectra, biological detection, and optical microscopy.

Programmable metasurfaces are revolutionizing the field of communication and perception by dynamically modulating properties such as amplitude and phase of electromagnetic (EM) waves. Nevertheless, it is challenging for existing programmable metasurfaces to attain fully independent dynamic modulation of amplitude and phase due to the significant correlation between these two parameters. In this paper, we propose a radiation-type metasurface that can realize radiation space-time coding of the joint amplitude-phase. Hence, independent and arbitrary modulation of amplitudes and phases can be achieved for both x-polarized and y-polarized EM waves. For demonstration, the dynamic beam scanning with ultra-low sidelobe levels (SLLs) is validated. Moreover, we propose a strategy of stochastic coding and non-uniform modulation to suppress the harmonic energy, thereby obtaining the ultra-low sideband levels (SBLs). Prototypes were fabricated and measured, and all simulations and measurements demonstrated the superiority of the proposed strategy. In addition, the proposed strategy is optimization-free and highly integrated, which has unrivaled potential in the field of compact communication systems and radar systems.

To adapt to the complex environment where low infrared emissivity and high infrared emissivity coexist, a radar stealth-infrared camouflage compatibility metasurface requires meta-atoms with customized infrared emissivity. Generally, the infrared emissivity is determined by the occupation ratio. However, the high occupation ratio will interfere with the scattering reduction function due to the Lorentz resonance from the metal patch. To address the problem, a method for decoupling Lorentz resonance is proposed in this paper. By shifting the resonant frequency of the metal patch to a high frequency, the Lorentz resonance is suppressed in the frequency band of scattering reduction. To verify the method, a single functional layer metasurface with microwave scattering reduction and customized infrared emissivity is designed. The scattering reduction at 3.5–5.5 GHz is realized through the polarization conversion. Meanwhile, the infrared emissivity of the metasurface can be gradient-designed by changing the occupation ratios of the meta-atoms. Compared with the initial design, the improved metasurface expands the infrared emissivity range from 0.60–0.80 to 0.51–0.80, and the scattering reduction effect remains unchanged. The experimental results agree with the simulated results. The work enriches the infrared emissivity function, which can be applied to camouflage in complex spectrum backgrounds.

Metasurfaces offer innovative approaches for manipulating electromagnetic waves at subwavelength scales. Recent advancements have focused on toroidal dipole (TD) and quasi-bound state in the continuum (quasi-BIC) modes, which are particularly attractive due to their capacity to enhance light-matter interaction. However, most metasurfaces with TD and quasi-BIC modes exhibit passive electromagnetic responses after fabrication, limiting their practical applications. This study presents both numerical and experimental investigations that demonstrate the active control of TD and quasi-BIC modes through the integration of symmetric and asymmetric aluminum dumbbell aperture arrays with the phase-change material Ge2Sb2Te5 (GST). The symmetric hybrid dumbbell aperture array shows a pronounced TD response within the terahertz frequency range. In contrast, modifying the geometric parameters to disrupt the structural symmetry induces a quasi-BIC mode in the asymmetric hybrid dumbbell aperture array. Furthermore, as GST undergoes a phase transition from its amorphous to crystalline state, both TD and quasi-BIC modes become dynamically tunable, driven by changes in the conductivity of GST. Notably, significant modulation of the transmitted terahertz wave occurs around the frequencies corresponding to the TD and quasi-BIC modes during the GST phase transition. Symmetric and asymmetric hybrid dumbbell aperture arrays provide a versatile platform for generating tunable TD and quasi-BIC modes, with promising applications in terahertz modulators and filters.

Imaging in the solar blind ultraviolet (UV) region offers significant advantages, including minimal interference from sunlight, reduced background noise, low false-alarm rate, and high sensitivity, and thus has important applications in early warning or detection of fire, ozone depletion, dynamite explosions, missile launches, electric leakage, etc. However, traditional imaging systems in this spectrum are often hindered by the bulkiness and complexity of conventional optics, resulting in heavy and cumbersome setups. The advent of metasurfaces, which use a two-dimensional array of nano-antennas to manipulate light properties, provides a powerful solution for developing miniaturized and compact optical systems. In this study, diamond metalenses were designed and fabricated to enable ultracompact solar-blind UV imaging. To prove this concept, two representative functionalities, bright-field imaging and spiral phase contrast imaging, were demonstrated as examples. Leveraging diamond’s exceptional properties, such as its wide bandgap, high refractive index, remarkable chemical inertness, and high damage threshold, this work not only presents a simple and feasible approach to realize solar-blind imaging in an ultracompact form but also highlights diamond as a highly capable material for developing miniaturized, lightweight, and robust imaging systems.

A reconfigurable metasurface based on optical control provides a control paradigm for integrating multiple functions at the same aperture, which effectively expands the freedom of control. However, the traditional light control method requires the light source to directly illuminate the photosensitive device, which forces the metasurface to be placed only according to the light emitter position, and even to need to be integrated on the light emitter, limiting the application scenarios of light-controlled reconfigurable metasurfaces. In this work, a light control method based on optical fiber is proposed, which guides and controls the light propagation path through optical fiber. The metasurface can be flexibly deployed, breaking through the limitation of physical space. As a verification, photoresistors are embedded in the metasurface, and the active device is directly excited by the light source as a driving signal to realize the switching of a polarization conversion function. The experimental results show that the optical-fiber-controlled metasurface can achieve linear-to-linear polarization conversion in the light environment and linear-to-circular polarization conversion in the dark environment. This work paves a new way, to our knowledge, to achieve a light-controlled metasurface, which enriches the family of intelligent metasurfaces and has great potential in many fields.

The finding of Snell’s law for anomalous reflection enables broad applications of metasurfaces in stealth, communication, radar technology, etc. However, some unavoidable high-order modes are inherently generated due to the super lattice of this local approach, which thus causes a decrease in efficiency and a limit in the reflected angle. Here, a novel, to our knowledge, low-profile wideband reflective meta-atom shaped like a four-leaf rose is proposed to achieve a phase coverage of full 360° by varying the length of the rose leaf. Then, the genetic algorithm is adopted for the first time to encode and optimize the topology of each meta-atom on the coding metasurface to achieve two-dimensional (2D) anomalous reflection with excellent performances through an inverse design. Numerical results show that our optimized coding metasurfaces achieve a high-efficiency (≥90%) and large-angle (θ≤70° and 0°≤φ≤360°) reflection under normal incidence. For verification, far-field measurement is carried out and experimental results are consistent with the numerical ones. Our work sets up a solid platform for utilizing algorithms, especially in artificial intelligence, in the future for arbitrary 2D anomalous reflection with high efficiency and a large angle.

Moiré meta-devices facilitate continuous and precise modulation of optical properties through the alteration of the relative alignment, such as twisting, sliding, or rotating of the metasurfaces. This capability renders them particularly suitable for dynamic applications, including zoom optics and adaptive imaging systems. Nevertheless, such designs often sacrifice more complex functionalities, such as polarization manipulation, in favor of simplicity and tunability. Here, we propose and experimentally validate a design strategy for a twisted bilayer metasurface that exhibits both varifocal capabilities and polarization filtering properties. By selecting silicon pillars with polarization-maintaining properties for Layer I and polarization-converting properties for Layer II, the designed Moiré metasurface can become sensitive to specific polarization states. Experimental results demonstrate that the proposed design can generate on-demand terahertz (THz) focused beams, achieving an average focusing efficiency exceeding 35% under x-linearly polarized (x-LP) illumination. This is accomplished by systematically varying the twisting angles p and q of Layer I in relation to Layer II in increments of 30°. Additionally, we provide numerical evidence that the focal length of the transmitted vortex beam can be adjusted using the same approach. The Moiré meta-device platform, which is engineered to modulate optical properties via mechanical twisting, obviates the necessity for external power sources or active materials. This generalized design strategy has the potential to significantly expedite the commercialization of multifunctional metasurfaces, which can produce high-precision optics across various practical applications.

In modern science and technology, on-demand control of the polarization and wavefront of electromagnetic (EM) waves is crucial for compact opto-electronic systems. Metasurfaces composed of subwavelength array structures inject infinite vitality to shape this fantastic concept, which has fundamentally changed the way humans engineer matter–wave interactions. However, achieving full-space arbitrarily polarized beams with independent wavefronts in broadband on a single metasurface aperture still remains challenging. Herein, the authors propose a generic method for broadband transmission-reflection-integrated wavefronts shaping with multichannel arbitrary polarization regulation from 8 to 16 GHz, which is based on the chirality effect of full-space non-interleaved tetrameric meta-molecules. Through superimposing eigen-polarization responses of the two kinds of enantiomers, the possibility for high-efficiency evolution of several typical polarization states with specific wavefronts is demonstrated. As proofs-of-concept, the feasibility of our methodology is validated via implementing miscellaneous functionalities, including circularly polarized (CP) beam splitting, linearly polarized (LP) vortex beams generation, and CP and LP multifoci. Meanwhile, numerous simulated and experimental results are in excellent agreement with the theoretical predictions. Encouragingly, this proposed approach imaginatively merges broadband polarization and phase control into one single full-space and shared-aperture EM device, which can extremely enhance the functional richness and information capacity in advanced integrated systems.

Metallic nanostructures supporting surface plasmons are crucial for various ultrathin photonic devices. However, these applications are often limited by inherent metallic losses. Significant efforts have been made to achieve high quality-factor (Q-factor) resonances in plasmonic metasurfaces, particularly through surface lattice resonances (SLRs) and bound states in the continuum (BICs). Despite these advances, a direct comparison between these two mechanisms remains unexplored. Here, we report a reusable plasmonic metasurface that supports multiple high-Q resonances by leveraging hybrid plasmonic–photonic modes. By systematically tuning the lattice constant and dielectric cladding thickness, we achieve substantial Q-factor enhancements of both SLRs and BICs in a monolithic device with a small footprint of 200 μm×200 μm by using an incoherent light source. A direct comparison between these two resonances is also discussed. This high-Q performance holds significant promise for applications in sensing, lasing, and nonlinear and quantum optics, paving the way for the development of next-generation nanophotonic devices.

Transition metal dichalcogenides (TMDs) hold great promise as a platform for optoelectronic devices, thanks to their exceptional optical characteristics. Nonetheless, their intrinsic low radiative recombination rate results in diminished efficiency in light emission and absorption. Here, we report photoluminescence (PL) enhancement of monolayer MoS2 through the utilization of full-wavelength (λ) nanodipole antennas. It is revealed that λ antennas demonstrate more pronounced PL enhancement and enhanced directivity compared to the previously examined half-wavelength (λ/2) antennas, relaxing the fabrication difficulty for ultra-narrow antenna gap configurations. By geometry and dimension optimization, a maximum PL enhancement of 17-fold is achieved. Furthermore, dual-polarized cross-shaped nanoantennas are developed to mitigate the reliance of the nanoantenna’s performance on the polarization state. Our method charts an effective path for amplifying the PL intensity of monolayer TMDs, thereby accelerating their integration into high-performance optoelectronic technologies.

The ultralow limit of detection (LoD) and exceptional sensitivity of biosensors are a significant challenge currently faced in the field. To address this challenge, this work proposes a highly sensitive laser ring cavity biosensor capable of detecting low concentrations of des-γ-carboxy prothrombin (DCP). A tapered W-shaped fiber probe based on multi-mode fiber (MMF)-multi-core fiber (MCF)-MMF is developed to excite strong evanescent waves (EWs). By immobilizing gold nanorods (GNRs) on the fiber probe, localized surface plasmon resonance (LSPR) is generated at the near infrared wavelength to further enhance the sensitivity of the fiber probe. Moreover, an erbium-doped fiber (EDF) ring laser with a narrow full width at half maximum (FWHM) of 0.11 nm is employed as a light source. The spectrum with narrow FWHM has been demonstrated to obtain lower LoD. Compared to the ASE light source, the LoD of the laser ring cavity can be reduced by an order of magnitude. The developed biosensor is capable of detecting DCP within a concentration range of 0–1000 ng/mL, and the detection sensitivity of 0.265 nm/lg(ng/mL) and the LoD of 367.6 pg/mL are obtained. In addition, the proposed laser ring cavity biosensor demonstrates good specificity, reproducibility, and repeatability by corresponding tests. The study results indicate that the proposed biosensor has potential in the detection of hepatocellular carcinoma markers.

In the food production sector, quickly identifying potential hazards is crucial due to the resilience of many pathogens, which could lead to wasted production results and, more severely, epidemic outbreaks. E. coli monitoring is essential; however, traditional quality control methods in fish farming are often slow and intrusive, thus promoting an increase in fish stress and mortality rates. This paper presents an alternative method by utilizing a prototype inspired by polarized optical microscopy (POM), constructed with a Raspberry Pi microprocessor to assess pixel patterns and calculate analyte levels. The sensors are based on the immune complexation reactions between E. coli specific antibodies and the disruption of liquid crystal (LC) alignment, which are measured with the POM technique. The prototype yielded a sensitivity of 1.01%±0.17%/log10 (CFU/mL) for E. coli. In this paper, tests using sunlight as the prototype’s light source were also performed, and a user-friendly graphical user interface was designed.

With the deepening integration of artificial intelligence (AI) and the Internet of Things (IoT) in daily life, electromagnetic sensing presents both attraction and increasing challenges, especially in the diversification, accuracy, and integration of sensing technologies. The remarkable ability of metasurfaces to manipulate electromagnetic waves offers promising solutions to these challenges. Herein, an integrated system for electromagnetic sensing and beam shaping is proposed. Improved genetic algorithms (GAs) are employed to design the metasurface with desired beams, while spatial electromagnetic signals sensitized by the metasurface are input into the GA enhanced by deep neural networks to sense the number of targets, their azimuths, and elevations. Subsequently, the metasurface device is designed as the hybrid mode combining tracking and avoidance in alignment with practical requirements and sensing outcomes. Simulation and experimental results validate the efficiency and accuracy of each module within the integrated system. Notably, the target sensing module demonstrates the capability to precisely sense more than 10 targets simultaneously, achieving an accuracy exceeding 98% and a minimum angular resolution of 0.5°. Our work opens, to our knowledge, a new avenue for electromagnetic sensing, and has tremendous application potential in smart cities, smart homes, autonomous driving, and secure communication.

Owing to the dynamic tunability and strong confinement, graphene plasmons (GPs) have emerged as an excellent candidate for the manipulation of light–matter interaction. Surface plasmons (SPs) have been admitted as another effective way allowing strong confinement of light at the nanoscale. The combination of GPs and SPs like localized surface plasmons (LSPs) and propagating surface plasmon polaritons (SPPs) will lead to a synergistic effect that could remarkably improve light–matter interactions, showing great potential for many applications for the improvement of solar cell efficiency, biosensor sensitivity, and the performance of photonic devices. In this study, the GPs were activated by placing graphene film onto a two-dimensional (2D) phase-changing crystalline Ge2Sb1.5Bi0.5Te5 (cGSBT) nanograting structure, which also acts as an original source generating LSPs. The SPPs originated by laying the above structure onto an Au mirror. The combined effects of GPs, LSPs, and SPPs are epitomized in such a simple Gr/2D cGSBT gratings/Au heterostructure, which allows easy realization of an ultrafast mode-locked laser quite stable working at 1550 nm range due to the strong nonlinear optical absorption capability. This approach overcomes the heat and energy loss in metallic gratings or a Gr-based heterostructure, exhibiting great potential for applications in the design and fabrication of photonic devices.

Vector vortex beams (VVBs) have garnered significant attention in fields such as photonics, quantum information processing, and optical manipulation due to their unique optical properties. However, traditional metasurface fabrication methods are often complex and costly, limiting their practical application. This study successfully fabricated an all-dielectric aluminum oxide metasurface capable of achieving longitudinal variation using 3D printing technology. Experimental results demonstrate that this metasurface generates longitudinally varying VVBs at 0.1 THz, with detailed characterization of its longitudinal intensity distribution and vector polarization states. The high consistency between experimental and simulation results validates the effectiveness of 3D printing in metasurface fabrication. The proposed metasurface offers promising applications in optical polarization control and communication, providing, to our knowledge, new insights and technical support for related research.

Surface plasmons (SPs) are one of the most effective information carriers for on-chip systems due to their two-dimensional propagation properties. Benefitting from the highly flexible designability, metasurfaces have emerged as a promising route in realizing SP devices. However, related studies are mainly focused on passive devices. Here, by introducing nonvolatile phase-change material Ge2Sb2Te5 (GST) into the metasurface design, we experimentally demonstrate a dual-function switchable SP device in the terahertz regime. Specifically, the device works as a spin-dependent directional plane-wave SP coupler when GST is in the amorphous state, while it works as a spin-dependent directional SP Fresnel zone plate (FZP) when GST is in the crystalline state. The states of GST are switched back and forth using thermal excitation and nanosecond laser illumination, respectively. Our method is simple and robust, and can find broad applications in on-chip photonic devices.

Recently organic-inorganic perovskite has been established as a promising platform for achieving room temperature exciton-polaritons, attributable to its superior optical coherence and robust exciton binding energies. However, when interfaced with metallic surfaces, the rapid degradation and quenching effect in perovskite have presented significant challenges, which critically hinders the exploration of light-matter interactions within metallic plasmonic structures. In this study, we report a quasi-two-dimensional lead halide perovskite that demonstrates a pronounced strong coupling phenomenon within an array of aluminum nanocones. The investigated quasi-two-dimensional perovskite structure exhibits high photoluminescence quantum efficiency and improved stability against metallic-induced degradation. Interestingly, the periodical arraying in honeycomb formation of plasmonic structure has advantages in angle-dependent dispersions and the loss neutralizing effectively. Besides, the plasmonic cone lattice characterized by its collective surface lattice resonance, features an exceptionally small mode volume and high quality, enhancing its interaction with the perovskite. A significant Rabi splitting of 243 meV is observed at an incident angle of 30°. The dynamics of the Rabi oscillation is revealed by transient absorption spectra and theoretically analyzed by cavity quantum electrodynamics. This advancement in polariton research paves the way for novel applications, including quantum sources, enhanced photon-electron conversion efficiencies, and low-threshold lasing.

Artificially designed hyperbolic metamaterials (HMMs) with extraordinary optical anisotropy can support highly sensitive plasmonic sensing detections, showcasing significant potential for advancements in medical research and clinical diagnostics. In this study, we develop a gold nanoridge HMM and disclose the plasmonic sensing physical mechanism based on this type of HMM through theoretical and experimental studies. We determine that the high modal group velocity of plasmonic guided modes stemming from a large transverse permittivity of HMMs directly results in high sensitivity. By combining electron-beam lithography, oxygen plasma etching, and electroplating, the fabricated gold nanoridge array possesses an extremely high structural filling ratio that is difficult to obtain through conventional processes. This leads to a large transverse permittivity and enables highly confined and ultra-sensitive bulk plasmon–polariton (BPP) guided modes. By exciting these modes in the visible to near-infrared region, we achieve a record sensitivity of 53,300 nm/RIU and a figure of merit of 533. Furthermore, the developed plasmonic nanoridge HMM sensor exhibits an enhanced sensitivity of two orders of magnitude compared to that of the same type of HMM sensor in label-free biomolecule detection. Our study not only offers a promising avenue for label-free biosensing but also holds great potential to enhance early disease detection and monitoring.

The dynamic and integrated control of near- and far-field electromagnetic waves is essential for advancing emerging intelligent information technology. Metasurfaces, distinguished by their low-profile design, cost-effectiveness, and ease of fabrication, have successfully revolutionized various electromagnetic functions. However, current research on the dynamic integrated manipulation of near-field and far-field electromagnetic waves using a single metasurface remains relatively constrained, due to the complexity of element-level control, restricted dynamic tuning range, and tuning speed. Herein, we propose an element-level controlled, versatile, compact, and broadband platform allowing for the real-time electronic reconstruction of desired near/far-field electromagnetic wavefronts. This concept is achieved by precisely regulating the 1-bit amplitude coding pattern across a guided-wave-excited metasurface aperture loaded with PIN diodes, following our binary-amplitude holographic theory and modified Gerchberg–Saxton (G–S) algorithm. Consistent findings across calculations, simulations, and experiments highlight the metasurface’s robust performance in 2D beam scanning, frequency scanning, dynamic focusing lens, dynamic holography display, and 3D multiplexing holography, even under 1-bit control. This simplified and innovative metasurface architecture holds the promise of substantially propelling forthcoming investigations and applications of highly integrated, multifunctional, and intelligent platforms.

Optical trapping has revolutionized various scientific disciplines with its non-invasive, high-resolution manipulation capabilities. However, conventional optical tweezers face limitations in effectively manipulating metallic particles due to their high reflectivity and associated scattering forces. Plasmonic tweezers, harnessing surface plasmons in metallic nanostructures, offer a promising solution by confining light to deep subwavelength scales and enhancing optical forces. However, dynamically manipulating metallic particles with plasmonic tweezers without mechanical adjustments remains a significant challenge. In this paper, we propose a novel approach utilizing dynamic optical tweezers with tunable plasmonic fields for metallic particle manipulation. By dynamically tailoring plasmonic fields with holograms, metallic particles can be manipulated without mechanical adjustments. Finite-difference time-domain simulations and Maxwell stress tensor calculations demonstrate the effectiveness of this technique, which offers simplicity, precision, and motionlessness in metallic particle manipulation. This advancement holds promise for applications in surface-enhanced Raman scattering, biosensing, super-resolved detection, and nanoparticle assembly, opening new avenues in plasmonic tweezers technology.

Ultrathin plasmonic nanostructures offer an unparalleled opportunity for the study of light–matter interactions at the nanoscale and realization of compact nanophotonic devices. In this study, we introduce an ultrathin gold nanoribbon array and demonstrate an electric approach to actively tuning its plasmonic resonance, which leveraging the extreme light confinement capability in the ultrathin plasmonic nanostructure and a robust nanoscale electro-optical effect in indium tin oxide. Optimizing the design (to a total thickness as small as 12 nm for a 2-nm-thick gold nanoribbon array), we numerically demonstrate a spectral shift in the plasmonic resonance up to 36 nm along with an approximately 16% change in the transmission at a gate voltage below 1.7 V at the wavelength of 1.47 μm. This work presents progress towards electric tuning of plasmonic resonances in ultrathin metallic nanostructures for various applications including surface-enhanced spectroscopy, spontaneous emission enhancement, and optical modulation.

Optical tweezers (OTs) can immobilize and manipulate objects with sizes that span between nano- and micro-meter scales. The manipulating ability of OTs is traditionally characterized by stability factor (S), which can only indicate an empirical “hit-or-miss” process. Additionally, the current quantitative models for trapping stability rarely consider the influence of external flow. In this paper, a comprehensive analysis to quantify the optical trapping stability in a perturbed asymmetric potential well is presented from the perspective of statistics, especially for weak trapping scenarios. Our analytical formulation takes experimentally measurable parameters including particle size, optical power, and spot width as inputs and precisely outputs a statistically relevant mean trapping time. Importantly, this formulation takes into account general and realistic cases including fluidic flow velocity and other perturbations. To verify the model, a back-focal-plane-interferometer-monitored trapping experiment in a flow is set up and the statistical characteristics of trapping time demonstrate good agreement with theoretical predictions. In total, the model quantitatively reveals the effects of external disturbance on trapping time, which will find applications where optical trapping stability is challenged by external perturbations in weak trapping conditions.

The consumption of contaminated food may cause serious illnesses, and traditional methods to detect Escherichia coli are still associated with long waiting times and high costs given the necessity to transport samples to specialized laboratories. There is a need to develop new technologies that allow cheap, fast, and direct monitoring at the site of interest. Thus, in this work, we developed optical immunosensors for the selective detection of E. coli, based on liquid crystal technology, whose molecules can align in different manners depending on the boundary conditions (such as substrates) as well as the environment that they experience. Each glass substrate was functionalized with anti-E. coli antibody using cysteamine as an intermediate, and a vertical alignment was imposed on the liquid crystal molecules by using DMOAP during functionalization. The presence of bacteria disrupts the alignment of the liquid crystal molecules, changing the intensity of light emerging between cross polarizers, measured using a polarized optical microscope and a monochromator. It was possible to detect E. coli in suspensions in the concentration range from 2.8 cells/mL to 2.8×109 cells/mL. Selectivity was also evaluated, and the sensors were used to analyze contaminated water samples. A prototype was developed to allow faster, in-situ, and easier analysis avoiding bulky instruments.

Topological photonics provides a platform for robust energy transport regardless of sharp corners and defects. Recently, the frequency multiplexing topological devices have attracted much attention due to the ability to separate optical signals by wavelength and hence the potential application in optical communication systems. Existing frequency multiplexing topological devices are generally based on the slow light effect. However, the resulting static local spatial mode or finely tuned flat band has zero-group velocity, making it difficult for both experimental excitation and channel out-coupling. Here, we propose and experimentally demonstrate an alternative prototype of asymmetric frequency multiplexing devices including a topological rainbow and frequency router based on floating topological edge mode (instead of localized ones); hence the multiple wavelength channels can be collectively excited with a point source and efficiently routed to separate output ports. The channel separation in our design is achieved by gradually tuning the band gap truncation on a topological edge band over a wide range of frequencies. A crucial feature lies in that the topological edge band is detached from bulk states and floating within the upper and lower photonic band gaps. More interestingly, due to the sandwiched morphology of the edge band, the top and bottom band gaps will each truncate into transport channels that support topological propagation towards opposite directions, and the asymmetrical transportation is realized for the frequency multiplexing topological devices.

Surface plasmon resonance (SPR) sensors are among the most sensitive sensors. In such devices, a grating is a compelling alternative to a prism for the excitation of a surface plasmon, especially in the development of sensors for point-of-care applications due to their compactness and cost-effectiveness. Here, we demonstrate the use of a tunable laser in a grating-based SPR system for further miniaturization and integration. The tunable laser working at normal incidence replaces spectral and moving components, while also simplifying the optical setup. Normal incidence is conventionally avoided due to the complexity of the control of degenerated SPR modes. We investigate, both computationally and experimentally, the splitting of the SPR modes at small nonzero incidences, which is lacking in previously reported studies. By optimizing the grating configuration, we were able to diminish the SPR mode splitting phenomenon when the excitation was feasible with the normal incidence configuration. The fabricated sensor showed a high sensitivity of 1101.6 nm/RIU. Notably, the figure of merit of the sensor, defined as the ratio between the sensitivity and bandwidth of the SPR dip, was 229.5. The experimental results were consistent with the simulation results. We also demonstrate its capability for detecting low concentrations of glucose and creatinine with the limit of detection of 14.2 and 19.1 mmol/L, respectively.

The narrowband meta-absorbers exhibit significantly enhanced electromagnetic confinement capabilities, showcasing broad application prospects in sensing fields. They can be applied for biomarker detection, chemical composition analysis, and monitoring of specific gas in the environment. In this work, we propose a 3D meta-absorber with an out-of-plane plasma mechanism based on a two-photon printing system. Compared to the conventional fabrication of a metal-insulator-metal 2D meta-absorber, the 3D absorber is composed of a metal layer and a resin layer from top to bottom; its manufacturing process is simpler, only including two-photon printing and magnetron sputtering deposition. A noticeable absorbing resonance appears at 0.3142 THz with perfect absorbance with a high Q-factor of 104.67. The theoretical sensitivity to the refractive index of the sensor reaches up to 172.5 GHz/RIU, with a figure of merit (FOM) of 19.56. In the experiments, it was validated as a meta-absorber with high sensitivity for doxycycline (DCH). As the DCH concentration increases from 0 to 4 mg/mL, the absorption intensity decreases around 49%, while the resonant frequency shift is around 70 GHz. It reflects the real-time residual content of DCH, and is potentially applied in trace antibiotic detection. The results showcase a perfect narrowband absorption capability with strong electromagnetic confinement in the terahertz spectrum, along with high-Q sensing characteristics of DCH. Compared to 2D metamaterials, the diversity of 3D metamaterial significantly expands, and introduces additional effects to provide greater flexibility in manipulating electromagnetic waves. The 3D device offers opportunities for the application of terahertz biochemical sensing.

Coding metasurfaces can manipulate electromagnetic wave in real time with high degree of freedom, the fascinating properties of which enrich the metasurface design with a wide range of application prospects. However, most of the coding metasurfaces are designed based on external excitation framework with the wired electrical or wireless light control devices, thus inevitably causing the interference with electromagnetic wave transmission and increasing the complexity of the metasurface design. In this work, a simplistic framework of single-pixel-programmable metasurfaces integrated with a capsuled LED array is proposed to dynamically control electromagnetic wave. The framework fully embeds the photoresistor in the meta-atom, controlling the LED array to directly illuminate the photoresistor to modulate the phase response. With this manner, the complex biasing network is transformed to the universal LED array, which means the physical control framework can be transformed to a software framework, and thus the functions of the metasurface can be freely manipulated by encoding the capsuled LED array avoiding mutual coupling of adjacent meta-atoms in real time. All the results verify that the far-field scattering pattern can be customized with this single-pixel-programmable metasurface. Encouragingly, this work provides a universal framework for coding metasurface design, which lays the foundation for metasurface intelligent perception and adaptive modulation.

The terahertz regime is widely recognized as a fundamental domain with significant potential to address the demands of next-generation wireless communications. In parallel, mode division multiplexing based on orbital angular momentum (OAM) shows promise in enhancing bandwidth utilization, thereby expanding the overall communication channel capacity. In this study, we present both theoretical and experimental demonstrations of an on-chip terahertz OAM demultiplexer. This device effectively couples and steers seven incident terahertz vortex beams into distinct high-quality focusing surface plasmonic beams, and the focusing directions can be arbitrarily designated. The proposed design strategy integrates space-to-chip mode conversion, OAM recognition, and on-chip routing in a compact space with subwavelength thickness, exhibiting versatility and superior performance.

Lead-free perovskite Cs2AgBiBr6 manifests great potential in developing high-performance, environmentally friendly, solution-processable photodetectors (PDs). However, due to the relatively large energy bandgap, the spectrum responses of Cs2AgBiBr6 PDs are limited to the ultraviolet and visible region with wavelengths shorter than 560 nm. In this work, a broadband Cs2AgBiBr6 PD covering the ultraviolet, visible, and near infrared (NIR) range is demonstrated by incorporating titanium nitride (TiN) nanoparticles that are prepared with the assistance of self-assembled polystyrene sphere array. In addition, an atomically thick Al2O3 layer is introduced at the interface between the Cs2AgBiBr6 film and TiN nanoparticles to alleviate the dark current deterioration caused by nanoparticle incorporation. As a result, beyond the spectrum range where Cs2AgBiBr6 absorbs light, the external quantum efficiency (EQE) of the TiN nanoparticle incorporated Cs2AgBiBr6 PD is enhanced significantly compared with that of the control, displaying enhancement factors as high as 2000 over a broadband NIR wavelength range. The demonstrated enhancement in EQE arises from the photocurrent contribution of plasmonic hot holes injected from TiN nanoparticles into Cs2AgBiBr6. This work promotes the development of broadband solution-processable perovskite PDs, providing a promising strategy for realizing photodetection in the NIR region.

Polarization is crucial in various fields such as imaging, sensing, and substance detection. A compact, fast, and accurate polarization detection device is vital for these applications. Herein, we demonstrate a multifocus metalens for terahertz polarization detection that requires only a single measurement to obtain complete polarization parameters and reconstruct the polarization state of the incident field. The individual subarrays of this metalens convert each of the six polarized components into the same polarization, which in turn links the Stokes parameters to these six foci. The incident linear polarizations and elliptical polarizations are characterized by Stokes parameters and polarization ellipses. Simulations and experimental results show that the scheme can accurately detect the incident polarization with a single measurement. The proposed metasurface polarimetry may find applications in the fields of real-time terahertz detection and integrated optics.

The coupling between surface plasmons and excitons in transition metal dichalcogenides (TMDs) plays crucial roles in light emission, nonlinear optics, and quantum information processing. However, the intermediate plasmon–exciton coupling has not been reported in the TMD-integrated metallic nanoarray. Herein, we demonstrate the intermediate coupling behavior between surface plasmons in the silver nanogroove array and excitons in 2D layered tungsten disulfide (WS2). The results show that the reflection spectra of the silver nanogroove array possess an obvious reflection dip at the wavelength of ∼630 nm due to the generation of surface plasmons. The experiment results are well consistent with the numerical simulations. When the silver nanoarray is integrated with a trilayer WS2, there exists a distinct coupling between surface plasmons and A excitons in WS2. The temporal coupled-mode theory analysis shows that the plasmon–exciton coupling locates in the intermediate plasmon–exciton coupling region. The intermediate coupling can give rise to the strong photoluminescence (PL) enhancement of 48-fold in WS2. The wavelength of the PL peak presents a red shift with the increase of the temperature. This work paves a new pathway for the generation of plasmon–exciton coupling and the PL enhancement in atomic-layer TMDs.

Hyperbolic phonon polaritons (HPhPs) in van der Waals layered polar crystals exhibit extreme light confinement capability, providing an unprecedented research opportunity to manipulate nanoscale midinfrared photons. Precise tuning of HPhPs propagation characteristics and near-field energy routing is crucial for applying polaritonic devices. Here, we demonstrate a widely tunable waveguide mode of HPhPs in an α-MoO3 flake/gold slit composite structure. By varying the width of the gold slit from 3 μm to 220 nm, the compression ratio of HPhPs wavelength relative to the incident light wavelength can be adjusted from 35% to 8.6%, respectively. This is attributed to the introduction of the gold slit, which can effectively excite and guide HPhPs within an α-MoO3 flake, forming a confined waveguide mode. Notably, the excitation efficiency of HPhPs in the nanoscale ultranarrow waveguide can be enhanced by integrating an extended port at the waveguide port. In addition, the routing of polaritons in a Y-shaped waveguide is realized by modulating the frequency of the incident light. This work presents a promising platform for manipulating deep subwavelength polaritons in planar photonic devices for infrared applications.

The exceptional point (EP), a degenerate point within non-Hermitian parametric space, has attracted considerable attention, especially for its chiral responses. However, achieving ideal circular dichroism (CD) remains challenging due to the existence of parallel components at the EP. Here, we delve into the theoretical condition required to attain a zero-transmission parallel component. This condition, together with the chiral EP condition, leads to a point characterized by near-unity CD, termed the super chiral EP (SCEP). To illustrate our theoretical framework, we introduce a parity-time symmetric metasurface with gain and loss. The observation of SCEP is demonstrated by tuning both the coupling strength and gain–loss ratio. Furthermore, we explore distinctive properties of SCEP, including phase flip and unidirectional invisibility. Leveraging SCEP and the topological phase transition point, we achieve polarization states across the entire Poincaré surface. This work opens avenues for potential applications in polarizing optical elements, holography, logic gates, chiral molecular detection, ultrasensitive sensing, and polarization-sensitive imaging.

Reconfigurable metasurfaces enable dynamic and real-time manipulation of electromagnetic (EM) waves in subwavelength resolution, possessing unparalleled potentials to construct meta-devices. However, most existing reconfigurable metasurfaces either operate under single polarization or in limited polarization channels or discretely tailor EM variables within relatively narrow bandwidth, which are hard to adapt to the urgent development requirements of multitask and highly integrated intelligent communication systems. Herein, a reconfigurable metasurface strategy based on continuous amplitude modulation utilizing circularly polarized (CP) basis vectors is proposed and demonstrated, with which the orthogonal component energy proportion of an arbitrarily polarized wave can be tailored, achieving full-polarization customized broadband and versatile function generation and control. Two symmetrically positive–intrinsic–negative diodes embedded into split-ring resonators are employed to simultaneously and independently switch dual-channel co-polarized amplitude with almost unaltered phase, which significantly simplifies control framework and enhances information capacity. In addition, a full-polarization reconfigurable metasurface prototype of 0.1λ0 thickness is designed and fabricated, which can continuously tune the reflection, polarization conversion, and absorption via loading different external bias voltages from 6 to 8.6 GHz. This inspiring methodology opens up routes for advanced multiplexed equipment and might find applications in future-oriented data storage and multi-input/multi-output systems.

Conversion from free-space waves to surface plasmons has been well studied as a key aspect of plasmonics. In particular, efficient coupling and propagation of surface plasmons via phase gradient metasurfaces are of great current research interest. Hereby, we demonstrate a terahertz metacoupler based on a bilayer bright–dark mode coupling structure attaining near-perfect conversion efficiency (exceeding 95%) without considering absorption loss of the materials and maintaining a high conversion level even when the area of the excitation region changes. To validate our design, a fabricated metacoupler was assessed by scanning near-field terahertz microscopy. Our findings could pave the way for developing high-performance plasmonic devices encompassing ultra-thin and compact functional devices for a diverse range of applications, especially within the realm of high-speed terahertz communications.

Single-pixel imaging is a burgeoning computational imaging technique that utilizes a single detector devoid of spatial resolution to capture an image, offering great potential for creating cost-effective and simplified imaging systems. Nevertheless, achieving super-resolution with a single pixel remains a formidable challenge. Here, we introduce a single-pixel super-resolution imaging technique based on space–time modulation. The modulation parametrically mixes the incoming signals, enabling the space–time scattered signals of the object carrying finer details to be captured by the single-pixel imaging system. To validate our proposed technique, we designed and fabricated a computational metasurface imager that needs only a single transmitting port and a single receiving port. The achieved resolution surpasses the Abbe resolution limit. The principle of our proposed technique is well-suited for low-cost and compact imaging systems.

In this paper, the concept of anisotropic impedance holographic metasurface is proposed and validated by realizing holographic imaging with multipoint focusing techniques in near-field areas at the radio frequency domain. Combining the microwave holographic leaky-wave theory and near-field focusing principle, the mapped geometrical patterns can be constructed based on the correspondence between meta-atom structural parameters and equivalent scalar impedances in this modulated metasurface. Different from conventional space-wave modulated holographic imaging metasurfaces, this surface-wave-based holographic metasurface fed by monopole antenna embedded back on metal ground enables elimination of the misalignment error between the air feeding and space-wave-based metasurface and increase of the integration performance, which characterizes ultra-low profile, low cost, and easy integration. The core innovation of this paper is to use the classical anisotropic equivalent surface impedance method to achieve the near-field imaging effect for the first time. Based on this emerging technique, a surface-wave meta-hologram is designed and verified through simulations and experimental measurements, which offers a promising choice for microwave imaging, information processing, and holographic data storage.

Nanoparticle-based plasmonic optical fiber sensors can exhibit high sensing performance, in terms of refractive index sensitivities (RISs). However, a comprehensive understanding of the factors governing the RIS in this type of sensor remains limited, with existing reports often overlooking the presence of surface plasmon resonance (SPR) phenomena in nanoparticle (NP) assemblies and attributing high RIS to plasmonic coupling or waveguiding effects. Herein, using plasmonic optical fiber sensors based on spherical Au nanoparticles, we investigate the basis of their enhanced RIS, both experimentally and theoretically. The bulk behavior of assembled Au NPs on the optical fiber was investigated using an effective medium approximation (EMA), specifically the gradient effective medium approximation (GEMA). Our findings demonstrate that the Au-coated optical fibers can support the localized surface plasmon resonance (LSPR) as well as SPR in particular scenarios. Interestingly, we found that the nanoparticle sizes and surface coverage dictate which effect takes precedence in determining the RIS of the fiber. Experimental data, in line with numerical simulations, revealed that increasing the Au NP diameter from 20 to 90 nm (15% surface coverage) led to an RIS increase from 135 to 6998 nm/RIU due to a transition from LSPR to SPR behavior. Likewise, increasing the surface coverage of the fiber from 9% to 15% with 90 nm Au nanoparticles resulted in an increase in RIS from 1297 (LSPR) to 6998 nm/RIU (SPR). Hence, we ascribe the exceptional performance of these plasmonic optical fibers primary to SPR effects, as evidenced by the nonlinear RIS behavior. The outstanding RIS of these plasmonic optical fibers was further demonstrated in the detection of thrombin protein, achieving very low limits of detection. These findings support broader applications of high-performance NP-based plasmonic optical fiber sensors in areas such as biomedical diagnostics, environmental monitoring, and chemical analysis.

Surface plasmons have been given high expectations in terahertz (THz) on-chip photonics with highly bound integrated transmission and on-chip wavefront engineering. However, most surface plasmonic coupling strategies with tailorable polarization-dependent features are challenged in broadband propagation and dynamic manipulation. In this work, a liquid crystal (LC)-integrated surface plasmonic metadevice based on arc-arrayed pair-slit resonators (APSRs) is demonstrated. The mirror-symmetry structures of this metadevice achieve the spin-selective unidirectional achromatic focusing, of which the broadband characteristic is supported by containing multiple APSRs with slits of different sizes corresponding to different excitation frequencies. Moreover, arc radii are precisely designed to meet the phase matching condition of constructive interference, so that the operating frequency of this on-chip metadevice is broadened to 0.33–0.60 THz. Furthermore, the LC integration provides the active energy distribution between the left and right focal spots, and the actual modulation depth reaches up to 73%. These THz active, wideband, on-chip manipulation mechanisms and their devices are of great significance for THz-integrated photonic communication, information processing, and highly sensitive sensing.

Programmable hyper-coded holography has the advantage of being programmable as well as being flexibly modifiable. Digitally coded metamaterials with excellent electromagnetic modulation capability and the ability to control the phase to modulate the spatial radiation field through external excitation in the form of switching can be used to realize low-cost digital arrays. We design a 1-bit encoded programmable metasurface, which is electrically connected to control the PIN diode in the switching state and to switch the condition of each metasurface cell between “0” and “1.” Using the designed programmable metasurface, we can randomly encode the cell structure to realize single-focus focusing, multi-focusing, and simple holographic letter imaging. Based on the nonlinear holographic model, we employ the Gerchberg-Saxton improvement algorithm to modulate the energy distribution at the focus by adjusting the phase distribution. Importantly, we introduce the Fourier convolution principle to regulate the holographic imaging focus flexibly.

Optical antennas have received considerable attention in recent years due to their unique ability to convert localized energy to freely propagating radiation and vice versa. Sidelobe level (SLL) is one of the most crucial parameters in antenna design. A low SLL is beneficial to minimize the antenna interference with other optical components. Here a plasmonic optical leaky-wave antenna with low SLL is reported. Shifting spatial frequency by periodically modulating the electric-field amplitude in a plasmonic gap waveguide enables a free-space coupled wave out of the antenna. At the same time, precise control of the aperture fields by the modulation depth allows for reducing SLL. Simulation results indicate that the proposed design can achieve a high directivity of 15.8 dB and a low SLL of -20 dB at the wavelength of 1550 nm. A low SLL below -15 dB is experimentally demonstrated within the wavelength range from 1527 to 1570 nm. In addition, the low-SLL property is further verified by comparing it with a uniformly modulated antenna. By modulating the guided waves in the plasmonic gap waveguide in different forms, the aperture fields can be flexibly arranged to achieve arbitrary wavefront shaping. It bridges the gap between guided and free-space waves and empowers plasmonic integrated devices to control free-space light, thus enabling various free-space functions.

Structured light carrying orbital angular momentum (OAM) opens up a new physical dimension for studying light–matter interactions. Despite this, the complex fields created by OAM beams still remain largely unexplored in terms of their effects on surface plasmons. This paper presents a revelation of anomalous plasmon excitations in single particles and plasmon couplings of neighboring nanorods under OAM beams, which are forbidden using non-OAM sources. The plasmon excitation of single nanoparticles is determined both by photon spin angular momentum (SAM) and OAM and influenced by the locations of the nanoparticles. Specifically, when SAM and OAM are equal in magnitude and opposite in direction, a pure plasmon excitation along light propagation direction is achieved. Two plasmon dipoles show end-to-end antibonding coupling and side-by-side bounding coupling, which are the opposite of the typical couplings. Furthermore, we observe Fano resonance with a nanorod dimer: one aligned along light propagation direction acting as the bright mode and the other aligned along the global polarization direction of light acting as the dark mode, which is the opposite of the usual plasmonic Fano resonance. By taking advantage of the unique property of the OAM source, this investigation presents a novel way to control and study surface plasmons, and the research of plasmon behavior with OAM would open new avenues for controlling electromagnetic waves and enriching the spectroscopies with more degrees of freedom.

Graphene-based terahertz (THz) metasurfaces combined with metallic antennas have the advantages of ultra-small thickness, electrical tunability, and fast tuning speed. However, their tuning ability is limited by non-independently tunable pixels and low modulation depth due to the ultra-small thickness of graphene. Here, we demonstrate a reconfigurable THz phase modulator with 5×5 independently tunable units enabled by switching the voltages applied on 10 graphene ribbons prepared by laser cutting. In addition, by introducing quasi-bound states in the continuum resonance through a designed double C-shaped antenna, the efficiency of the device is enhanced by 2.7–3.6 times under different graphene chemical potentials. Experimental results demonstrate that a focus can be formed, and the focal length is changed from 14.3 mm to 22.6 mm. This work provides potential for compact THz spatial light modulators that may be applied in THz communication, detection, and imaging.

Chiral mirrors can produce spin selective absorption for left-handed circularly polarized (LCP) or right-handed circularly polarized (RCP) waves. However, the previously proposed chiral mirror only absorbs the designated circularly polarized (CP) wave in the microwave frequency band, lacking versatility in practical applications. Here, we propose a switchable chiral mirror based on a pair of PIN diodes. The switchable chiral mirror has four working states, switching from the handedness-preserving mirror to the LCP mirror, RCP mirror, and perfect absorber. The basis of these advances is to change the chirality of two-dimensional (2D) chiral metamaterials and the circular conversion dichroism related to it, which is the first report in the microwave frequency band. Surface current distributions shed light on how switchable chiral mirrors work by handedness-selective excitation of reflective and absorbing electric dipole modes. Energy loss distributions verify the working mechanism. The thickness of the switchable chiral mirror is one-tenth of the working wavelength, which is suitable for integrated manufacturing. The measurement results are in good agreement with the simulation results.

Fifth-generation (5G) communication requires spatial multiplexing multiple-input multiple-output systems with integrated hardware. With the increase in the number of users and emergence of the Internet of Things devices, complex beamforming devices have become particularly important in future wireless systems to meet different communication requirements, where independent amplitude and phase modulations are urgently required for integrated beamforming devices. Herein, by utilizing the constructive interference between multiple geometric-phase responses, the mathematical relation for decoupling amplitude and phase modulations in the radiation-type operational mode is derived. Based on this strategy, complex-amplitude radiation-type metasurfaces (RA-Ms) are implemented, with an integrated feeding network. Such metasurfaces exploit full 2π phase modulation and tailorable radiation amplitude in the circular polarization state. Meanwhile, a complex-amplitude retrieval method is developed to design the RA-Ms, enabling precise beamforming performances. On this basis, several functional devices based on the complex-amplitude RA-Ms, including energy-allocable multi-router, shape-editable beam generator, and complex beamformer, are demonstrated in the microwave region. The amplitude-phase decoupling mechanism with the retrieval method merges amplitude and phase modulations, and energy distribution into one compact and integrated electromagnetic component and may find applications in multi-target detection, 5G mobile communication, and short-range ground-to-sea radar.

Metasurfaces have intrigued long-standing research interests and developed multitudinous compelling applications owing to their unprecedented capability for manipulating electromagnetic waves, and the emerging programmable coding metasurfaces (PCMs) provide a real-time reconfigurable platform to dynamically implement customized functions. Nevertheless, most existing PCMs can only act on the single polarization state or perform in the limited polarization channel, which immensely restricts their practical application in multitask intelligent metadevices. Herein, an appealing strategy of the PCM is proposed to realize tunable functions in co-polarized reflection channels of orthogonal circularly polarized waves and in co-polarized and cross-polarized reflection channels of orthogonal linearly polarized waves from 9.0 to 10.5 GHz. In the above six channels, the spin-decoupled programmable meta-atom can achieve high-efficiency reflection and 1-bit digital phase modulation by selecting the specific ON/OFF states of two diodes, and the phase coding sequence of the PCM is dynamically regulated by the field-programmable gate array to generate the desired function. A proof-of-concept prototype is constructed to verify the feasibility of our methodology, and numerous simulation and experimental results are in excellent agreement with the theoretical predictions. This inspiring design opens a new avenue for constructing intelligent metasurfaces with higher serviceability and flexibility, and has tremendous application potential in communication, sensing, and other multifunctional smart metadevices.

Directionally scattered surface plasmon polaritons (SPPs) promote the efficiency of plasmonic devices by limiting the energy within a given spatial domain, which is one of the key issues to plasmonic devices. Benefitting from the magnetic response induced in high-index dielectric nanoparticles, unidirectionally scattered SPPs have been achieved via interference between electric and magnetic resonances excited in the particles. Yet, as the magnetic response in low-index dielectric nanoparticles is too weak, the directionally scattered SPPs are hard to detect. In this work, we demonstrate forward scattered SPPs in single low-index polystyrene (PS) nanospheres. We numerically illustrate the excitation mechanism of plasmonic induced electric and magnetic multipole modes, as well as their contributions to forward SPP scattering of single PS nanospheres. We also simulate the SPP scattering field distribution obtaining a forward-to-backward scattering intensity ratio of 50.26:1 with 1 μm PS particle. Then the forward scattered SPPs are experimentally visualized by Fourier transforming the real-space plasmonic imaging to k-space imaging. The forward scattered SPPs from low-index dielectric nanoparticles pave the way for SPP direction manipulation by all types of nanomaterials.

Bound states in continuum (BICs) are believed to have the ability to achieve high quality factor (Q factor) resonances, which is very important for plasmonics. However, the study of plasmonic BICs is not sufficient. Herein, we design and fabricate a metal-insulator-metal (MIM) metasurface and demonstrate a one-dimensional plasmonic BIC experimentally. The even-order localized surface plasmon resonance (LSPR) modes have even parity at normal incidence. The symmetry-protected BIC can be achieved at Γ point. The band structure can be tuned by strong coupling between the localized plasmonic resonance and plasmonic lattice mode. Interestingly, two of the hybrid modes are also BICs. Although BICs cannot interact with the far field, we successfully demonstrate BIC splitting through far-field excitation. By further tuning the pitch of the MIM grating, the Friedrich–Wintgen BIC is also observed. Finally, we propose and preliminarily demonstrate an ultrathin bandpass spatial filter. These findings provide a new platform to study optical multipole BICs and can have applications in fields such as nano lasers, ultrasensitive sensors, filters, nonlinearity enhancement, and quantum optics.

High-performance terahertz (THz) devices with reconfigurable features are highly desirable in many promising THz applications. However, most of the existing reconfigurable THz elements are still limited to volatile responses, single functionality, and time-consuming multistep manufacturing procedures. In this paper, we report a lithography-free approach to create reconfigurable and nonvolatile THz components by exploring the reversible, nonvolatile, and continuous THz modulation capability of the phase change material Ge2Sb2Te5. As a proof of concept, THz gratings with significant Rayleigh anomalies and diffraction as well as ultrathin THz flat lenses with subwavelength and ultra-broadband focusing capabilities are designed and fabricated on ultrathin Ge2Sb2Te5 films using the presented photo-imprint strategy. Moreover, such a method can also be adopted to create more complex THz devices, such as Pancharatnam–Berry phase metasurfaces and grayscale holographic plates. With these findings, the proposed method will provide a promising solution to realize reconfigurable and nonvolatile THz elements.

We present octave-wide bandpass filters in the terahertz (THz) region based on bilayer-metamaterial (BLMM) structures. The passband region has a super-Gaussian shape with a maximum transmittance approaching 70% and a typical stopband rejection of 20 dB. The design is based on a metasurface consisting of a metallic square-hole array deposited on a transparent polymer, which is stacked on top of an identical metasurface with a subwavelength separation. The superimposed metasurface structures were designed using finite-difference time-domain (FDTD) simulations and fabricated using a photolithography process. Experimental characterization of these structures between 0.3 and 5.8 THz is performed with a time-domain THz spectroscopy system. Good agreement between experiment and simulation results is observed. We also demonstrated that two superimposed BLMM (2BLMM) devices increase the steepness of the roll-offs to more than 85 dB/octave and enable a superior stopband rejection approaching 40 dB while the maximum transmittance remains above 65%. This work paves the way toward new THz applications, including the detection of THz pulses centered at specific frequencies, and an enhanced time-resolved detection sensitivity toward molecular vibrations that are noise dominated by a strong, off-resonant, driving field.

Compared to pure vortex waves, the superposition state of spherical waves and vortex waves has enough degrees of freedom to upgrade applications in particle manipulation, information encryption, and large-capacity communications. Here, we propose a new scheme to achieve superposition states and multichannel transmission of vortex and spherical waves. Two transmissive all-silicon metasurfaces that enable mutual interference between linearly polarized (LP) waves in the terahertz region are demonstrated. Type A can achieve interference between x and y polarized waves, while type B can achieve interference between x (or y) and x (or y) polarized waves. The multichannel transmission and superposition states of topological charges of +3, +2, and +4 are designed and demonstrated from theoretical, simulative, and experimental perspectives at 1.1 THz. In addition, the objective fact that the focused superposition state must be observed close to the focal plane is also revealed. The measured results are in good agreement with the theoretical and simulative results. This work provides an idea for the design of ultrathin terahertz devices and could be applied in the fields of information encryption and high-frequency communications.

Plasmonic resonances empowered by bound states in the continuum (BICs) offer unprecedented opportunities to tailor light–matter interaction. However, excitation of high quality-factor (Q-factor) quasi-BICs is often limited to collimated light at specific polarization and incident directions, rendering challenges for unpolarized focused light. The major hurdle is the lack of robustness against weak spatial coherence and poor polarization of incident light. Here, addressing this limitation, we demonstrate sharp resonances in symmetric plasmonic metasurfaces by exploiting BICs in the parameter space, offering ultraweak angular dispersion effect and polarization-independent performance. Specifically, a high-Q (≈71) resonance with near-perfect absorption (>90%) is obtained for the input of unpolarized focused light covering wide incident angles (from 0° to 30°). Also, giant electric and magnetic field enhancement simultaneously occurs in quasi-BICs. These results provide a way to achieve efficient near-field enhancement using focused light produced by high numerical aperture objectives.

Metasurfaces have great potential for flexible manipulation of electromagnetic wave polarizations and wavefronts. Here, we propose a general method for achieving independent wavefront manipulation in a single polarization-multiplexing transmissive metasurface. As a proof of concept, we design a transmission-type anisotropic metasurface for independent wavefront manipulation in full-polarization channels. An x-polarized wave transmitted through such a metasurface could be converted into four outgoing beams with delicately designed polarization states that converge to specific positions for holographic imaging. The measured results are in good agreements with simulated ones, verifying the independent wavefront manipulations with arbitrary polarization conversions. Compared with the existing traditional meta-devices with single-polarization modulation, we achieve polarization-multiplexed metasurfaces with mixed polarization and phase control, which can greatly improve the functional richness of the system.

The manipulation and detection of polarization states play a crucial role in the application of 6G terahertz communication. Nonetheless, the development of compact and versatile polarization detection devices capable of detecting arbitrary polarizations continues to be a challenging endeavor. Here, we demonstrate a terahertz polarization detection scheme by performing mode purity analysis and multidimensional analysis of the transmitted vortex field. The power of the proposed polarization recognition is verified by using three polarization trajectories, including linear polarizations, circular polarizations, and elliptical polarizations. Using the reconstructed complete polarization parameters, the detected polarization states are characterized using polarization ellipses, Poincaré sphere, and full-Stokes parameters. The experimental results validate the power of this scheme in polarization detection. This scheme holds promise for applications in polarization imaging and terahertz communication.

Surface lattice resonance (SLR) is a pretty effective mechanism to realize ultranarrow linewidths in the spectrum. Herein, we propose and demonstrate reflection-type SLRs in all-metal metasurfaces experimentally, compared with the traditional transmission-type SLR, which can avoid the refractive index (RI) mismatch problem and are more suitable for high-efficiency RI sensing due to direct contact and strong light–matter interaction. The measured SLR linewidth is 13.5 nm influenced by the meta-atom size, which needs a compromise design to keep a balance between the narrow linewidth and noise immunity. Notably, the SLR sensitivity is determined by the lattice period along the polarization direction with regularity, which establishes an intuitive link between structures and optical responses and provides a theoretical guide for metasurface designs. Additionally, incident angle multiplexing will make the resonance wavelength red shift or blue shift in the case of orthogonal polarization. The rectangular array metasurface can realize dual SLRs with different sensing performances. Flexibly, the SLR can also be formed by the different meta-atoms and arrays. This research supports SLR multifarious applications involving not only RI sensing but also nonlinear optics, nano-lasers, etc.

Surface lattice resonances (SLRs) with ultra-narrow linewidth (high quality factor) can enhance light–matter interactions at the nanoscale and modulate the propagating light from the emission wavelength direction to efficiency by photonic band engineering. Therefore, SLRs can serve as an excited candidate to enhance and, more importantly, modulate amplified spontaneous emission (ASE) with more optical parameters. Here, this work presents a system of two-dimensional Ag-coated Al nanocone array (Ag-NCA) packaged with Nile red, and a normal ASE with 15-fold enhancement is observed under external driving light. This enhancement fades away, obviously, in the case of the off-normal condition, as the optical feedback evolves from the band edge steady state to the propagating state. The ASE of this hybrid plasmonic system expands the possibilities of interaction between light and matter and has great promise for applications in nanolasing, super-resolution imaging, and photonic integration circuits.

Employing couplers to convert guided waves into free-space modes and flexibly control their wavefront is one of the key technologies in chip-integrated displays and communications. Traditional couplers are mainly composed of gratings, which have limitations in footprint, bandwidth, as well as controllability. Though the resonant/geometric metasurface newly emerges as a promising interface for bridging guided waves with free-space ones, it either relies on complex optimizations of multiple parameters, or is subject to the locked phase response of opposite spins, both of which hinder the functional diversity and practical multiplexing capability. Here, we propose and experimentally demonstrate an alternative with a spin-decoupled meta-coupler, simultaneously integrating triple functions of guided wave radiation, polarization demultiplexing, and dual-channel wavefront manipulation into a single device. By endowing polarization-dependent functionalities into a pure geometric metasurface, the out-coupled left-handed and right-handed circular polarization guided waves intelligently identify the predesigned phase modulation and reconstruct desired wavefronts, like bifocal focusing and holography multiplexing, with a polarization extinction ratio over 13.4 dB in experiments. We envision that the robust, broadband, and multifunctional meta-coupler could pave a way for the development of versatile multiplexed waveguide-based devices.

Optical frequency combs (OFCs) have great potential in communications, especially in dense wavelength-division multiplexing. However, the size of traditional OFCs based on conventional optical microcavities or dispersion fibers is at least tens of micrometers, far larger than that of nanoscale electronic chips. Therefore, reducing the size of OFCs to match electronic chips is of necessity. Here, for the first time to our knowledge, we introduce surface plasmon polaritons (SPPs) to the construction of OFCs to realize a miniature device. The thickness of our device is reduced below 1 μm. Though the presence of SPPs may induce ohmic and scattering loss, the threshold of the device is obtained as 9 μW, comparable to the conventional device. Interestingly, the response time is 13.2 ps, much faster than the optical counterparts. This work provides a feasible strategy for the miniaturization of OFCs.

Owing to their unique optical properties and new degrees of freedom, orbital angular momentum (OAM) beams have been applied in various fields. Detection of the topological charges (TCs) of OAM beams is the key step for their applications. However, on-chip sorting of OAM beams with large TCs still remains a challenge. In this paper, Bloch surface wave (BSW) structures with five semi-ring shaped nanoslits are modeled. A spatial separation of 135 nm on the chip is obtained between two neighboring OAM states. OAM beams with TCs up to 35 can be successfully sorted by the BSW structures, which is much larger than that using metallic structures (only seven). BSW structures exhibit better OAM sorting performances than metallic structures. We systematically show how the lower attenuation of BSW structures leads to far superior separation ability compared to surface plasmons propagating on metallic structures. In addition, sorting of two OAM beams with different TCs simultaneously can be achieved in this way. Our results reveal that BSW structures should be an excellent solution for OAM sorting with large TCs, which is beneficial for applications in integrated on-chip devices and optical communications.

With the rapid development of nanophotonics for enhancing free-electron radiation, bound states in the continuum (BICs) have emerged as a promising approach for emitting intense Smith–Purcell radiation (SPR) with enhanced intensity. However, current BIC-based methods are limited to single-frequency operation, thereby restricting their applications requiring spectral and angular tunability, such as particle detectors and light sources. To overcome this limitation, this work proposes an approach for constructing plasmonic BICs over a broad spectral range in symmetry-broken systems. By leveraging the high-Q resonances near the BICs, we achieve intense SPR with broadband tunability, potentially improving the radiation intensity by six orders compared to traditional methods. Experimentally, we validate the construction of BIC using plasmonic antennas and achieve broadband demonstration. Our proposed concept can be extended to other plasmonic or guided-wave systems, paving the way toward compact and efficient free-electron sources in hard-to-reach frequency regimes.

Recently, multifarious deformation approaches in nature have promoted dynamic manipulation for electromagnetic (EM) waves in metamaterials, and those representative strategies are mainly focused on the modulation of spectral parameters. Several works have also achieved tunable phase-gradient meta-devices. Here, to broaden the modulation freedom of mechanical deformation, we initially propose two reconfigurable metamaterials consisting of mirrored S-shaped meta-atoms selectively bonded on biaxially pre-stretched substrates. Planar meta-atoms with spin-insensitive transmittance are buckled into 3D morphologies to break residual symmetries by releasing the stress and to facilitate spin-dependent transmittance under circularly polarized incidence. Owing to the geometric anisotropy of S-shaped meta-atoms along the x and y axes, 3D chiral meta-atoms exhibit discriminate circularly cross-polarized transmittance under opposite spins. The underlying physical mechanism reveals that EM resonance originates from the excitation of electric dipoles and magnetic dipoles, and their cross coupling finally triggers the chiral effects of 3D meta-atoms. By introducing the gradient-phase design that keeps unchanged under various strains, two types of meta-atoms with specified orientations are interleaved to design a double-foci metalens, and its 2D-to-3D morphology transformation shortens the focusing length and facilitates the intensity change of two foci. Our approach in designing reconfigurable EM metamaterials with 2D-to-3D buckling transformability can be further extended toward terahertz even optical wavebands, and it may assist with deriving more applicable multi-functionalities in the aspects of imaging, sensing, and holograms.

Terahertz vortices prompt numerous advanced applications spanning classical and quantum communications, sensing, and chirality-based detection, owing to the inherent physical properties of terahertz waves and orbital angular momentum (OAM). Nonetheless, existing methodologies for generating terahertz vortices face challenges such as unalterable topological charges and intricate feed networks. To address these limitations, we propose a novel approach to generate multi-mode and tunable vortex beams based on chiral plasmons. Through eigenmode analysis, the uniform helical gratings are demonstrated to support chiral plasmons carrying OAM. By leveraging their vortex characteristics and introducing modulation into the periodic system, these chiral plasmons are alternatively diffracted into high-purity vortex radiations according to the Bragg law. To validate the theory, the vortex beam emitter is fabricated and measured in the microwave regime based on the modulated scheme. Experimental results confirm the emission of vortex beams with desirable phase distributions and radiation patterns. Our findings highlight the potential of chiral plasmons as seeds for tunable and compact vortex radiation, offering promising applications in tunable vortex sources.

Long-wave infrared (LWIR, 8–14 µm) photonics is a rapidly growing research field within the mid-IR with applications in molecular spectroscopy and optical free-space communication. LWIR applications are often addressed using rather bulky tabletop-sized free-space optical systems, preventing advanced photonic applications, such as rapid-time-scale experiments. Here, device miniaturization into photonic integrated circuits (PICs) with maintained optical capabilities is key to revolutionize mid-IR photonics. Subwavelength mode confinement in plasmonic structures enabled such miniaturization approaches in the visible-to-near-IR spectral range. However, adopting plasmonics for the LWIR needs suitable low-loss and -dispersion materials with compatible integration strategies to existing mid-IR technology. In this paper, we further unlock the field of LWIR/mid-IR PICs by combining photolithographic patterning of organic polymers with dielectric-loaded surface plasmon polariton (DLSPP) waveguides. In particular, polyethylene shows favorable optical properties, including low refractive index and broad transparency between ∼2 μm and 200 µm. We investigate the whole value chain, including design, fabrication, and characterization of polyethylene-based DLSPP waveguides and demonstrate their first-time plasmonic operation and mode guiding capabilities along S-bend structures. Low bending losses of ∼1.3 dB and straight-section propagation lengths of ∼1 mm, pave the way for unprecedented complex on-chip mid-IR photonic devices. Moreover, DLSPPs allow full control of the mode parameters (propagation length and guiding capabilities) for precisely addressing advanced sensing and telecommunication applications with chip-scale devices.

Optically transparent microwave absorbing metasurfaces have shown great potential and are needed in multiple applications environments containing optical windows owing to their ability to reduce backscattering electromagnetic (EM) signals while keeping continuous optical observation. Meanwhile, they are also required to have adaptive EM manipulation capability to cope with complex and capricious EM environments. As a general approach, distributed circuit components, including positive-intrinsic-negative diodes and varactors and sensing components, are integrated with passive absorbing metasurfaces to realize adaptive control of microwave absorption. However, these circuit elements generally require bulky electrical wires and complex control circuits to regulate the operating state, resulting in the absorbing structures being optically opaque. Hence, it is a great challenge to realize self-operating absorbers while maintaining optical transparency. Here, we report an optically transparent cognitive metasurface made of patterned graphene sandwich structures and a radio frequency detector, which can achieve adaptive frequency manipulation to match incident EM waves. As a proof-of-principle application example, we realize a closed-loop automatic absorber system prototype of the proposed graphene metasurface with self-adaptive frequency variation, without any human intervention. The approach may facilitate other adaptive metadevices in microwave regime with high-level recognition and manipulation and, more generally, promote the development of intelligent stealth technologies.

Metallic nanoplasmonics, due to its extremely small size and ultrafast speed, has been one of the key components for next-generation information technology. It is vital that the highly tunable nanoplasmonic system in the solid state can be achieved for optoelectronic devices, which, still remains elusive for the visible region. Here we sandwich vanadyl oxalate (VOC2O4) thin films in-between gold nanoparticles and gold film to establish thermo-responsive nanoantennas. The thickness of the VOC2O4 composite films remains almost unchanged within the temperature cycles between 15°C and 80°C, while the refractive index of the films decreases with the increase of temperature due to the dehydration, which results in blueshift of the plasmon peak up to 60 nm. The plasmon resonances can be fully recovered when the temperature cools down again. This process is reversible within the temperature range of 15°C–80°C, which can be optically modulated with photothermal effect. Such thermo-responsive plasmonic nanoantenna works in the solid state with hundreds of kilohertz switching speed, which is highly compatible with traditional optoelectronic devices. It can be envisioned that this thermo-responsive optical thin film can be a promising candidate for integrated nanoplasmonic and optoelectronic devices.

Aqueous solutions cannot be detected using transmissive terahertz metamaterials because water strongly absorbs terahertz waves. Transmissive terahertz metamaterials are easier to integrate terahertz emitters and receivers into single and compact devices than reflective terahertz metamaterials. The detection of aqueous solutions using transmissive terahertz metamaterials is a big challenge. This work fabricates a transmissive terahertz metamaterial using a folding metamaterial comprising split-ring resonators (SRRs) with nano-profiles with a high aspect ratio of 41.4. The folding metamaterial has a small transmittance of -49 dB at its resonance frequency, large transmittance contrast of approximately 6×104 with respect to the transmittance of its substrate, large refractive index sensitivity of 647 GHz/RIU, and large quality factor of 37. This result arises from the nano-profiles of the SRRs. The nano-profiles increase the surface areas of the SRRs, increasing their surface currents and enhancing the electromagnetic resonance of the folding metamaterial. The folding metamaterial detects a 188-μm-thick rabbit-blood layer that is deposited on it, which cannot be detected by using a common metamaterial. This result reveals that folding metamaterials have potential in detecting the products of live microorganisms with geometrical sizes up to several hundreds of micrometers, such as hydrogen gas, hydrocarbons, and antibodies.

The interaction between magnetic quantum emitters and the local electromagnetic environment is a promising method to manipulate the spontaneous emission. However, it is severely limited by the weak interactions between the magnetic component of light and natural materials. Herein, we demonstrate that the special type of anapole states associated with the “onefold” electric toroidal dipole moment can be excited by efficient interaction between magnetic dipole emitters and silver oligomers. Based on magnetic anapole states, the radiative power is effectively suppressed with significant coupling between the emitter and the silver nonamer, physically providing an ideal playground for the study of non-radiative transitions. These findings not only introduce magnetic anapoles to plasmonics but also open a door for the development of new high-performance magnetic-dipole-based optoelectronic devices.

Stainless steel is a basic raw material used in many industries. It can be customized by generating laser-induced periodic surface structure (LIPSS) as subwavelength gratings. Here, we present the capabilities of an LIPSS on stainless steel to modify the polarization state of the reflected radiation at the IR band. These structures have been modeled using the finite element method and fabricated by femtosecond laser processing. The Stokes parameters have been obtained experimentally and a model for the shape has been used to fit the simulated Stokes values to the experimental data. The birefringence of the LIPSS is analyzed to explain how they modify the polarization state of the incoming light. We find the geometry of the subwavelength grating that makes it work as an optical retarder that transforms a linearly polarized light into a circularly polarized wave. In addition, the geometrical parameters of the LIPSS are tuned to selectively absorb one of the components of the incoming light, becoming a linear axial polarizer. Appropriately selecting the geometrical parameters and orientation of the fabricated LIPSS makes it possible to obtain an arbitrary pure polarization state when illuminated by a pure linearly polarized state oriented at an azimuth of 45°. The overall reflectance of these transformations reaches values close to 60% with respect to the incident intensity, which is the same reflectivity obtained for non-nanostructured stainless steel flat surfaces.

Metasurfaces have powerful light field manipulation capabilities and have been researched and developed extensively in various fields. With an increasing demand for diverse functionalities, terahertz (THz) metasurfaces are also expanding their domain. In particular, integrating different functionalities into a single device is a compelling domain in metasurfaces. In this work, we demonstrate a functionally decoupled THz metasurface that can incorporate any two functions into one metasurface and switch dynamically through external excitation. This proposed metasurface is formed by the combination of split-ring resonators and phase change material vanadium dioxide (VO2). It operates in the single-ring resonant mode and double-ring resonant mode with varying VO2 in insulating and metallic states, respectively. More importantly, the phase modulation is independent in two operating modes, and both cover a 360° cross-polarized phase with efficient polarization conversion. This characteristic makes it obtain arbitrary independent phase information on the metasurface with different modes to switch dual functions dynamically. Here, we experimentally demonstrate the functions of a tunable focal length and large-angle focus deflection of a THz off-axis parabolic mirror to verify the dual-function switching characteristics of the functionally decoupled metasurface. The functionally decoupled metasurface developed in this work broadens the way for the research and application of multifunctional modulation devices in the THz band.

Plasmonic high-quality factor resonators with narrow surface plasmon resonance (SPR) linewidths are extremely significant for surface-enhanced Raman scattering, optical sensors, imaging, and color filters. Unfortunately, extensive research on narrowing SPR linewidths is mainly based on noble metal nanostructures that are restricted by intrinsic loss. Here, heterostructures consisting of metal and dielectric metaphotonics are experimentally designed and fabricated for elaborating SPR linewidths. The results demonstrate that the SPR linewidths can be narrowed by 66.7% relative to that of aluminum nanostructures. The resonant linewidths are directly shrunk due to the interaction between low loss in the semiconductor nanostructures and electromagnetic confinement in the metal counterparts. Meanwhile, the resonant wavelength governed by heterostructure configurations shifts from 600 to 930 nm. This work will pave an avenue toward controlling resonant linewidths of metal-dielectric heterostructures for numerous applications.

Approaches to generate and manipulate Cherenkov radiation (CR) are challenging yet meaningful. Optical topological transition (OTT) in novel materials and metamaterials is also promising for modern photonics. We study the OTT of CR in graphene-based hyperbolic metamaterials (GHMs) for the first time. In GHMs, conventional and hyperbolic CR can be switched when crossing the topological transition frequency. This frequency can be altered by metamaterial components and external optical elements. For instance, external ultrafast optical pumps cause an ultrafast OTT from the elliptical to the hyperbolic state. Then, hyperbolic CR can be excited by low-energy electrons by leveraging the excellent photothermal properties of graphene. Hyperbolic CR vanishes when the GHM returns to its original state. Furthermore, graphene nonlocality occurs when the electron velocity is low enough, corresponding to a large wave vector. Concretely, when the electron velocity approaches the Fermi velocity of graphene, a nonlocality-induced OTT modifies the plasmonic properties of the GHM and brings a new lower velocity threshold of hyperbolic CR. Therefore, hyperbolic CR can only be induced in a limited velocity range. These findings pave the way for understanding CR properties in active plasmonic metamaterials and may be applied to complex photonic and polaritonic systems.

The integration of nano-emitters into plasmonic devices with spatial control and nanometer precision has become a great challenge. In this paper, we report on the use of a smart polymer to selectively immobilize nano-emitters on specific preselected sites of gold nanocubes (GNCs). The cunning use of the polymer is twofold. First, it records both the selected site and the future emitters–GNC distance through plasmon-assisted photopolymerization. Second, because the polymer is chemically functionalized, it makes it possible to attach the nano-emitters right at the preselected polymerized sites, which subsequently recognize the nano-emitters to be attached. Since the resulting active medium is a spatial memory of specific plasmonic modes, it is anisotropic, making the hybrid nanosources sensitive to light polarization. The ability to adjust their statistical average lifetime by controlling the thickness of the nanopolymer is demonstrated on two kinds of nano-emitters coupled to GNCs: doped polystyrene nanospheres and semiconductor colloidal quantum dots.

The investigation of converged twisted beams with a helical phase structure has a remarkable impact on both fundamental physics and practical applications. Geometric metasurfaces consisting of individually orientated metal/dielectric meta-atoms provide an ultracompact platform for generating converged vortices. However, it is still challenging to simultaneously focus left-handed and right-handed circularly polarized incident beams with pure geometric phase modulation, which hinders the independent operation on topological charges between these two helical components. Here we propose and experimentally demonstrate an approach to design terahertz geometric metasurfaces that can generate helicity-independent converged vortices with homogeneous polarization states by the superposition of two orthogonal helical vortices with identical topological charges. Furthermore, the multiplexing of polarization-rotatable multiple vortices in multiple dimensions, i.e., in both longitudinal and transverse directions, and a vortex with an extended focal depth is confirmed by embedding polarization modulation into the geometric metasurfaces. The demonstrated approach provides a new way to simultaneously manipulate orthogonal helical components and expand the design dimension, enabling new applications of geometric metasurface devices in polarization optics, twisted-beam related image and edge detection, high capacity optical communication, and quantum information processing, to name a few.

Dual-focusing effect with a cylindrical vector-light characteristic (i.e., radial and azimuthal polarizations) is theoretically proposed and numerically demonstrated by spin-decoupled phase control with all-silicon metalens. Attributed to the polarization dependence, the pair of focusing cylindrical vector beams can be interchanged by orthogonally switching the polarization of incident light. We demonstrate the unique contributions of focused radial and azimuthal vector beams to longitudinal and transverse optical forces on glass spheres, respectively, by calculations based on the Maxwell stress tensor. This paper presents the use of all-silicon metalens with highly-compact vector beams, promising for applications such as multidimensional optical trapping.

The manipulation of high-quality vector beams (VBs) with metasurfaces is an important topic and has potential for classical and quantum applications. In this paper, we propose a Fresnel zone (FZ) metasurface with metallic nanoslits arranged on FZs, which sets alternate binary geometric and propagation phases to cancel the incident spin component and focus the converted spin component (CSC). The rotation designs of nanoslits transform the incident polarization state on the conventional Poincaré sphere to VBs on the higher-order Poincaré (HOP) sphere. The two orbital angular momentum states of the CSCs were manipulated, and the focused HOP beams were generated. The experimental results demonstrate the broadband generation of arbitrarily focused HOP beams of high quality under the illumination of the red (632.8 nm), green (532 nm), and blue (473 nm) light. This work will be of significance for the applications of VBs in different areas, such as precision metrology, optical micromanipulation, and quantum information.

Optical skyrmions, quasiparticles that are characterized by the topologically nontrivial vectorial textures of optical parameters such as the electromagnetic field, Stokes parameters, and spin angular momentum, have aroused great attention recently. New dimensions for optical information processing, transfer, and storage have become possible, and developing multiple schemes for manipulating the topological states of skyrmions, thus, is urgent. Here we propose an approach toward achieving dynamic modulation of skyrmions via changing the field symmetry and adding chirality. We demonstrate that field symmetry governs the skyrmionic transformation between skyrmions and merons, whereas material chirality modulates the twist degree of fields and spins and takes control of the Néel-type–Bloch-type skyrmionic transition. Remarkably, the enantioselective twist of skyrmions and merons results from the longitudinal spin arising from the chirality-induced splitting of the hyperboloid in the momentum space. Our investigation, therefore, acts to enrich the portfolio of optical quasiparticles. The chiral route to topological state transitions will deepen our understanding of light–matter interaction and pave the way for chiral sensing, optical tweezers, and topological phase transitions in quantum matter.

Reconfigurable metasurfaces have attracted a deal of attention owing to their multifunctional and dynamic electromagnetic (EM) manipulation properties. However, most of the previous reconfigurable metasurfaces rely on manual control for function switching, which has huge limitations in practical application. Here, an intelligent metasurface with the self-adaptively EM manipulation capability is proposed. It integrates the sensing-and-feedback components to construct a closed-loop system, which can automatically adjust EM functionalities for the different incident power information. The sensing module in this metasurface can first perceive the incident EM power intensity and then provide the feedback signal to the field programmable gate array controlling platform that can send the corresponding instruction to the executing material for switching the EM functionality among transmission, reflection, and tunable absorption. Good self-adaptive reaction capability and practicability of the proposed metasurface have been demonstrated by the experiment. It has the capability of making a real-time response with adaptive EM behavior to the varying incoming wave power without the aid of human beings. Our design provides an avenue toward intelligent and cognitive metasurfaces, which has extensive application prospects in smart skin, intelligent absorber, and the related EM fields.

We evaluate the sensing properties of plasmonic waveguide sensors by calculating their resonant transmission spectra in different regions of the non-Hermitian eigenmode space. We elucidate the pitfalls of using modal dispersion calculations in isolation to predict plasmonic sensor performance, which we address by using a simple model accounting for eigenmode excitation and propagation. Our transmission calculations show that resonant wavelength and spectral width crucially depend on the length of the sensing region, so that no single criterion obtained from modal dispersion calculations alone can be used as a proxy for sensitivity. Furthermore, we find that the optimal detection limits occur where directional coupling is supported, where the narrowest spectra occur. Such narrow spectral features can only be measured by filtering out all higher-order modes at the output, e.g., via a single-mode waveguide. Our calculations also confirm a characteristic square root dependence of the eigenmode splitting with respect to the permittivity perturbation at the exceptional point, which we show can be identified through the sensor beat length at resonance. This work provides a convenient framework for designing and characterizing plasmonic waveguide sensors when comparing them with experimental measurements.

We theoretically and experimentally demonstrate that magnetic plasmonic gradient metasurfaces (GMSs) can convert a spatially propagating wave to a one-way edge state or vice versa with high efficiency. Consisting of an array of ferrite rods with a rotation gradient introduced to the rod dimers in the unit cell, GMSs can covert an incident wave beam to a one-way edge state with efficiency over 77%, and almost fully radiate into free space from the one-way edge state. The phenomenon arises from the unidirectional coupling of the spatial electromagnetic wave with magnetic plasmonic GMSs, which is evidenced from the photonic band diagrams of the edge state. The one-way edge state can radiate to or be excited from air with different angles by either engineering the gradient of the GMSs or tuning the bias magnetic field. By designing magnetic plasmonic GMSs with more exquisite configurations, we can expect many more nonreciprocal properties, adding additional freedom in manipulating electromagnetic waves.

Integrated metasurfaces with diversified functionalities have demonstrated promising prospects for comprehensive implementations in compact 5G/6G communication systems by flexibly manipulating electromagnetic (EM) waves. Increasingly emerged multifunctional metasurfaces have successfully revealed integrated wavefront manipulations via phase gradient arrays, coding apertures, independent polarization control, asymmetric transmission/reflection, etc. However, multifunctional metasurfaces with more degrees of freedom in terms of multi-band/broadband operation frequencies, full-space coverage, and computable array factors are still in dire demand. As a step forward in extending manipulation dimensions, we propose and corroborate a dual-band multifunctional coding metasurface for anomalous reflection, radar cross-section reduction, and vortex beam generation through full-wave analysis and experiment. Our tri-layer meta-device comprises a shared coding aperture of split-ring and cross-shaped resonators sandwiched between two layers of orthogonal wire gratings. With an approach of independent control of a reflection–transmission wavefront under orthogonal polarization states and Fabry–Perot-like constructive interference, the low-cross-talk shared coding aperture features a smooth phase shift and high efficiency for 3-bit coding in the K-band and 1-bit coding in the Ka-band. Both numerical and measured results verify that the proposed coding metasurface can effectively realize full-space EM control and improve the capacity of the information channel, which could be developed for potential applications in multifunctional devices and integrated systems.

In this paper, we design and demonstrate a compact logic operator based on a single-layer metasurface at microwave frequency. By mapping the nodes in the trained fully connected neural network (FCNN) to the specific unit cells with phase control function of the metasurface, a logic operator with only one hidden layer is physically realized. When the incident wave illuminates specific operating regions of the metasurface, corresponding unit cells are activated and can scatter the incident wave to two designated zones containing logical information in the output layer. The proposed metasurface logic operator is experimentally verified to achieve three basic logic operations (NOT, OR, and AND) under different input signals. Our design shows great application potential in compact optical systems, low-power consumption information transmission, and ultrafast wave-based full signal processing.

Biosensors are a focus of research on terahertz metasurfaces. However, reports of ultra-sensitive biosensors based on Dirac points are rare. Here, a new terahertz metasurface is proposed that consists of patterned graphene and perovskites. This serves as an ultra-sensitive Dirac-point-based biosensor for qualitative detection of sericin. Theoretically, sericin may make graphene n-doped and drive the Fermi level to shift from the valence band to the Dirac point, causing a dramatic decrease in conductivity. Correspondingly, the dielectric environment on the metasurface undergoes significant change, which is suited for ultra-sensitive biosensing. In addition, metal halide perovskites, which are up-to-date optoelectronic materials, have a positive effect on the phase during terahertz wave transmission. Thus, this sensor was used to successfully detect sericin with a detection limit of 780 pg/mL, achieved by changing the amplitude and phase. The detection limit of this sensor is as much as one order of magnitude lower than that of sensors in published works. These results show that the Dirac-point-based biosensor is a promising platform for a wide range of ultra-sensitive and qualitative detection in biosensing and biological sciences.

Broadband absorbers generally consist of plasmonic cavities coupled to metallic resonators separated by a dielectric film, and they are vertically stacking configurations. In this work, we propose an ultra-broadband nanowire metamaterial absorber composed of an array of vertically aligned dielectric nanowires with coaxial metallic rings. The absorber shows strong absorption from 0.2 to 7 μm with an average absorption larger than 91% due to the excitation of gap surface plasmon polariton modes in Fabry–Perot-like resonators. Moreover, a refractory dielectric cladding can be added to improve the thermal stability of the absorber, showing a negligible impact on its absorption performance. The proposed absorber may find potential applications in solar energy harvesting, infrared imaging and spectroscopy, and optoelectronic devices.

Thermo-plasmonics, using plasmonic structures as heat sources, has been widely used in biomedical and microfluidic applications. However, a metasurface with single-element unit cells, considered as the sole heat source in a unit cell, functions at a fixed wavelength and has limited control over the thermo-plasmonically induced hydrodynamic effects. Plasmonic metasurfaces with metal disk heterodimer lattices can be viewed to possess two heat sources within a unit cell and are therefore designed to photo-actively control thermal distributions and fluid dynamics at the nanoscale. The locations of heat sources can be switched, and the direction of the convective flow in the central region of the unit cell can be reversed by shifting the wavelength of the excitation source without any change in the excitation direction or physical actuation of the structural elements. The temperature and velocity of a fluid are spatiotemporally controlled by the wavelength selectivity and polarization sensitivity of the plasmonic metasurface. Additionally, we investigate the effects of geometric parameters on the surface lattice resonances and their impact on the temperature and fluid velocity of the optofluidic system. Our results demonstrate excellent optical control of these plasmonic metasurface heating and thermal convection performances to design flexible platforms for microfluidics.

The spatial distribution of electromagnetic fields emitted from the aperture tip of a scanning near-field optical microscope (SNOM), which is called the emission pattern, depends on the geometry of the apex and the material composition of the tip’s coating. In previous works, experimental measurements of the emission pattern from the aperture tip were performed mostly in the far field. Moreover, the corresponding theoretical models were also developed based on these far-field measurements. Here, we have used the automated dual-tip SNOM to systematically characterize the emission from the aperture tip in the near field. In this regard, we have considered three different pairs of excitation and detection tips with distinct geometries. The emission patterns of the excitation tips were mapped using detection tips. Unidirectional surface plasmon polaritons (SPPs) at the surface of a gold platelet were launched by an excitation tip and measured in the near field by the detection tip. The experimental results were numerically reproduced by means of the Bethe–Bouwkamp model. This work puts into evidence the applicability of the automated dual-tip SNOM as the only available characterization technique to measure the emission from aperture tips in the near field. The reported asymmetric SPP radiation patterns can find applications in photonic integrated circuits or in biological and chemical sensing.

Active control of the electromagnetically induced transparency (EIT) analog is desirable in photonics development. Here, we theoretically and experimentally proposed a novel terahertz (THz) asymmetric metasurface structure that can possess high-sensitivity modulation under extremely low power density by integrating perovskite or graphene. Using the novel metasurface structure with the perovskite coating, the maximum amplitude modulation depth (AMD) of this perovskite-based device reached 490.53% at a low power density of 12.8037 mW/cm2. In addition, after the novel THz metasurface structure was combined with graphene, this graphene-based device also achieved high AMD with the maximum AMD being 180.56% at 16.312 mW/cm2, and its transmission amplitude could be electrically driven at a low bias voltage. The physical origin of this modulation was explained using a two-oscillator EIT model. This work provides a promising platform for developing high-sensitivity THz sensors, light modulators, and switches.

It is highly desirable to flexibly and actively manipulate the dephasing time of a plasmon in many potential applications; however, this remains a challenge. In this work, by using femtosecond time-resolved photoemission electron microscopy, we experimentally demonstrated that the Fano resonance mode in the asymmetric nanorod dimer can greatly extend the dephasing time of a femtosecond plasmon, whereas the non-Fano resonance results in a smaller dephasing time due to the large radiative damping, and flexible manipulation of the dephasing time can be realized by adjusting one of the nanorods in the Fano asymmetric dimer. Interestingly, it was found that plasmon resonance wavelengths both appeared red-shifted as the length of the upper or lower nanorods increased individually, but the dephasing time varied. Furthermore, it also indicated that the dephasing time can be prolonged with a smaller ascending rate by increasing the length of both the nanorods simultaneously while keeping the dimer asymmetry. Meanwhile, the roles of radiative and nonradiative damping in dephasing time are unveiled in the process of nanorod length variation. These results are well supported by numerical simulations and calculations.

Optical surface waves have widely been used in optical tweezers systems for trapping particles sized from the nano- to microscale, with specific importance and needs in applications of super-resolved detection and imaging if a single particle can be trapped and manipulated accurately. However, it is difficult to achieve such trapping with high precision in conventional optical surface-wave tweezers. Here, we propose and experimentally demonstrate a new method to accurately trap and dynamically manipulate a single particle or a desired number of particles in holographic optical surface-wave tweezers. By tailoring the optical potential wells formed by surface waves, we achieved trapping of the targeted single particle while pushing away all surrounding particles and further dynamically controlling the particle by a holographic tweezers beam. We also prove that different particle samples, including gold particles and biological cells, can be applied in our system. This method can be used for different-type optical surface-wave tweezers, with significant potential applications in single-particle spectroscopy, particle sorting, nano-assembly, and others.

Optical fiber surface plasmon resonance (SPR) sensors point toward promising application potential in the fields of biomarker detection, food allergen screening, and environmental monitoring due to their unique advantages. This review outlines approaches in improving the fiber SPR sensing performance, e.g., sensitivity, detection accuracy, reliability, cross-sensitivity, selectivity, convenience and efficiency, and corresponding sensing applications. The sensing principles of SPR sensors, especially the performance indicators and their influencing factors, have been introduced. Current technologies for improving the fiber SPR performance and their application scenarios are then reviewed from the aspects of fiber substrate, intrinsic layer (metal layer), and surface nanomaterial modification. Reasonable design of the substrate can strengthen the evanescent electromagnetic field and realize the multi-parameter sensing, and can introduce the in situ sensing self-compensation, which allows corrections for errors induced by temperature fluctuation, non-specific binding, and external disturbances. The change of the intrinsic layer can adjust the column number, the penetration depth, and the propagation distance of surface plasmon polaritons. This can thereby promote the capability of sensors to detect the large-size analytes and can reduce the full width at half-maximum of SPR curves. The modification of various-dimensionality nanomaterials on the sensor surfaces can heighten the overlap integral of the electromagnetic field intensity in the analyte region and can strengthen interactions between plasmons and excitons as well as interactions between analyte molecules and metal surfaces. Moreover, future directions of fiber SPR sensors are prospected based on the important and challenging problems in the development of fiber SPR sensors.

Plasmonic sensing based on nanostructures is a powerful analytical tool for ultrasensitive label-free biomolecule detection that holds great potential in the field of clinical diagnostics and biomedical research. Here, we report the fabrication, the characterization, and the principle of operation of gold nanorod hyperbolic metamaterials (NHMMs) along with ultrasensitive bulk refractive index and label-free biomolecular detection. By combining electron-beam lithography and nanoscale electroplating, we demonstrate the fabrication of a highly ordered, height-controllable, and vertical array of nanorods. By exciting the bulk plasmon–polariton mode in the NHMM using a prism-coupling technique and integrating the sensor in microfluidics, we demonstrate that the bulk sensitivity and figure of merit of our device could reach 41,600 nm/RIU and 416 RIU-1, respectively. The physical mechanism of this high bulk sensitivity is revealed through theoretical and experimental studies. Moreover, by bio-functionalizing the surface of the NHMM sensor, monitoring the binding of streptavidin at dilute concentrations is performed in real time. We test different concentrations of streptavidin ranging from 200 to 5 µg/mL, and the NHMM biosensor exhibits a 1 nm wavelength shift for a 5 µg/mL streptavidin detection. By fitting the Hill equation of the NHMM biosensor and taking into account the level of noise (0.05 nm) as the minimum wavelength shift of the detectable limit, the limit of detection of the NHMM biosensor to streptavidin can be estimated to be 0.14 µg/mL (2.4 nm). As a direct comparison, a 0.5 nm wavelength shift for 20 µg/mL of streptavidin is reported when using a conventional gold film sensor under identical experimental conditions. The developed plasmonic NHMM sensor shows tremendous potential for highly sensitive bulk solutions and biomolecule detection and provides a promising avenue for free-label biosensing applications in the future.

Surface plasmon resonance (SPR) sensors are a prominent means to detect biological and chemical analytes and to investigate biomolecular interactions in various fields. However, the performance of SPR sensors is ultimately limited by ohmic loss, which substantially weakens the resonance signal and broadens the response linewidth. Recent studies have shown that ohmic loss can be fully compensated in plasmonic nanolasers, which leads to a novel class of lasing-enhanced surface plasmon resonance (LESPR) sensors with improved sensing performance. In this paper, we detail the underlying physical mechanisms of LESPR sensors and present their implementation in various sensing devices. We review recent progress on their applications, particularly for refractive index sensing, gas detection and biological imaging, labeling, tracking, and diagnosis. We then summarize the review and highlight remaining challenges of LESPR sensing technology.

The in-plane negative refraction of high-momentum (i.e., high-k) photonic modes could enable many applications such as imaging, focusing, and waveguiding in a planar platform at deep-subwavelength scales. However, its practical implementation in experiments remains elusive so far. Here we propose a class of hyperbolic metasurfaces, which is characterized by an anisotropic magnetic sheet conductivity and can support the in-plane ultra-high-k magnetic designer polaritons. Based on such metasurfaces, we report the experimental observation of the all-angle negative refraction of designer polaritons at extremely deep-subwavelength scales. Moreover, we directly visualize the designer polaritons with hyperbolic dispersions. Importantly, for these hyperbolic polaritons, we find that their squeezing factor is ultra-large. To be specific, it can be up to 129 in the experiments, an ultra-high value exceeding those in naturally hyperbolic materials. This work may pave a way toward exploring the extremely high confinement and unusual propagation of magnetic designer polaritons over monolayer or twisted bilayer hyperbolic metasurfaces.

The integration of micro-electro-mechanical system (MEMS) with metamaterial has provided a novel route to achieve programmability via its reconfigurable capabilities. Here, we propose and demonstrate a MEMS-based metadevice by using switchable winding-shaped cantilever metamaterial (WCM) for active logical modulation. WCM can be actuated by external driving voltage, and the logical modulation bit is performed by releasing MEMS cantilevers to represent “on” and “off” states. While the underneath substrate surface of a MEMS-based metadevice is rough after releasing the cantilevers, the metadevice is allowed to operate on the reconfigurable switching state and avoid the snapping down of the device when the system is overloaded. Such a reconfigurable and programmable MEMS-based metadevice exhibits multifunctional characteristics to simultaneously perform the logic operations of “OR” and “AND” gates. By exploiting the tuning mechanism of the MEMS-based metadevice, the arbitrary metamaterial configuration can be implanted into WCM. This opens a wide avenue to further enlarge the operating frequency range and applications in optoelectronic fields. These unique results provide various possibilities in multifunctional switching, active logical modulating, and optical computing applications.

In this work, we present a novel biochemical sensing approach based on a plasmonic sensor chip, combined with a specific receptor, excited and interrogated via a custom 3D-printed holder through a transmission-based experimental setup, exploiting polymer optical fibers. The setup is designed to measure a disposable plasmonic chip based on a gold nanograting fabricated on a polymethylmethacrylate substrate. The examined sensor configurations here presented are simulated, realized, and experimentally tested. More specifically, first, a numerical analysis is carried out by changing several sensor parameters, then an experimental optical characterization of different sensor configurations is reported. Finally, to test the biosensing capabilities of the proposed method, as a proof of concept, we deposit on the best sensor configuration a biomimetic receptor specific for bovine serum albumin detection. The experimental results demonstrate that the proposed sensor shows an ultra-low limit of detection, equal to about 37 pmol/L.

Metasurface plays a key role in various terahertz metadevices, while the designed terahertz metasurface still lacks flexibility and variety. On the other hand, inverse design has drawn plenty of attention due to its flexibility and robustness in the application of photonics. This provides an excellent opportunity for metasurface design as well as the development of multifunctional, high-performance terahertz devices. In this work, we demonstrate that, for the first time, a terahertz metasurface supported by the electromagnetically induced transparency (EIT) effect can be constructed by inverse design, which combines the particle swarm optimization algorithm with the finite-difference time-domain method. Incorporating germanium (Ge) film with inverse-designed metasurface, an ultrafast EIT modulation on the picosecond scale has been experimentally verified. The experimental results suggest a feasibility to build the terahertz EIT effect in the metasurface through an optimization algorithm of inverse design. Furthermore, this method can be further utilized to design multifunctional and high-performance terahertz devices, which is hard to accomplish in a traditional metamaterial structure. In a word, our method not only provides a novel way to design an ultrafast all-optical terahertz modulator based on artificial metamaterials but also shows the potential applications of inverse design on the terahertz devices.

Strong coupling (SC) between two resonant plasmon modes can result in the formation of new hybrid modes exhibiting Rabi splitting with strong energy exchange at the nanoscale. However, normal Rabi splitting is often limited to ～50–320 meV due to the short lifetime of the plasmon mode. Here, we theoretically demonstrate a record Rabi splitting energy as large as 805 meV arising from the SC between the high-Q plasmonic whispering gallery mode and high-Q cavity plasmon resonance supported by a spherical hyperbolic metamaterial cavity, which consists of a dielectric nanosphere core wrapped in 7 alternating layers of silver/dielectric materials. In addition, the new hybrid modes formed by the SC are shown to exhibit an extralong lifetime of up to 71.9–81.6 fs, with the large electric field intensity enhancement at both the dielectric core and the dielectric layers. More importantly, the spectral ranges of SC can be tuned across an ultrabroad range from the visible to the near-IR by simply changing the dielectric core size. These findings may have potential applications in bright single-photon sources.

Anapole states, accompanied by strong suppression of light scattering, have attracted extensive attention in recent years due to their supreme performance in enhancing both linear and nonlinear optical effects. Although both low- and high-order anapole states are observed in the dielectric particles with high refractive index, so far few studies have touched on the topic of plasmonic anapole states. Here we demonstrate theoretically and numerically that the ideal plasmonic anapole states (strong suppression of electric dipole scattering) can be achieved in metallic metamolecules via increasing the coupling strength between Cartesian electric dipole and toroidal dipole moments of the system. The increasing coupling is based on compensation of ohmic losses in a plasmon system by introducing of a gain material, the influence of which is well described by the extended coupled oscillator model. Due to suppression of dipole radiation losses, the excitation of anapole states in plasmonic systems can result in enhancement of the near fields in subwavelength spatial regions outside of nanoparticles. That is especially important for developments of nonlinear nanophotonic and plasmonic devices and active functional metamaterials, which provide facilities for strong light energy concentration at the nanoscale. Development of the considered anapole effect with increase of metamolecule components is discussed.

Pixelated metasurfaces integrating both the functions of linear polarization and circular polarization filters on a single platform can achieve full-Stokes polarization detection. At present, the pixelated full-Stokes metasurfaces mainly face the following problems: low transmission, low circular dichroism (CD) of circular polarization filters, and high requirements in fabrication and integration. Herein, we propose high performance ultracompact all-dielectric pixelated full-Stokes metasurfaces in the near-infrared band based on silicon-on-insulator, which is compatible with the available semiconductor industry technologies. Circular polarization filters with high CD are achieved by using simple two-dimensional chiral structures, which can be easily integrated with the linear polarization filters on a single chip. In addition, the dielectric materials have higher transmission than metal materials with intrinsic absorption. We experimentally demonstrated the circular polarization filter with maximum CD up to 70% at a wavelength of 1.6 μm and average transmission efficiency above 80% from 1.48 μm to 1.6 μm. Therefore, our design is highly desirable for many applications, such as target detection, clinical diagnosis, and polarimetric imaging and sensing.

Chiral metasurfaces based on asymmetric meta-atoms have achieved artificial circular dichroism (CD), spin-dependent wavefront control, near-field imaging, and other spin-related electromagnetic control. In this paper, we propose and experimentally verify a scheme for achieving high-efficiency chiral response similar to CD of terahertz (THz) wave via phase manipulation. By introducing the geometric phase and dynamic phase in an all-silicon metasurface, the spin-decoupled terahertz transmission is obtained. The giant circular dichroism-like effect in the transmission spectrum is observed by using a random phase distribution for one of the circular polarization components. More importantly, the effect can be adjusted when we change the area of the metasurface illuminated by an incident terahertz beam. In addition, we also demonstrate the spin-dependent arbitrary wavefront control of the transmitted terahertz wave, in which one of the circularly polarized components is scattered, while the other forms a focused vortex beam. Simulated and experimental results show that this method provides a new idea for spin selective control of THz waves.

Ultrafast spatiotemporal control of a surface plasmon polariton (SPP) launch direction is a prerequisite for ultrafast information processing in plasmonic nanocircuit components such as ultrafast on–off of plasmonic switching and information recording. Here we realize for the first time, to the best of our knowledge, ultrafast spatiotemporal control of the preferential launch direction of an SPP at the nano-femtosecond scale via a plasmonic nano directional coupler. The spatiotemporal switching of the SPP field was revealed using time-resolved photoemission electron microscopy (TR-PEEM). Experimental results show that the extinction ratio of the SPP directional coupler can be substantially optimized by properly selecting the amplitude and time delay of the two incident light pulses in the experiment. More importantly, we demonstrate a solution for the launch direction of the SPP field, switched in a plasmonic nano directional coupler on the femtosecond timescale, by adjusting the instantaneous polarization state of the excitation light. The TR-PEEM images are supported by finite-difference time-domain (FDTD) simulations. We believe the results of this study can be used to develop high-speed, miniaturized signal processing systems.

Plasmonic particle-on-film nanocavities, supporting gap modes with ultra-small volume, provide a great solution to boost light–matter interactions at the nanoscale. In this work, we report on the photoluminescence (PL) enhancement of monolayer MoS2 using high order modes of an Au nanosphere dimer-on-film nanocavity (DoFN). The high order plasmon modes, consisting of two bonding quadrupoles in the dimer and their images in the Au film, are revealed by combining the polarization-resolved scattering spectra with the numerical simulations. Further integrating the monolayer MoS2 into the DoFN, these high order modes are used to enhance PL intensity through simultaneously boosting the absorption and emission processes, producing a 1350-fold enhancement factor. It opens an avenue to enhance the light–matter interaction with high order plasmon modes and may find applications in future optoelectronics and nanophotonics devices.

Chiral optical responses of bilayer metasurfaces made of twisted metallic nanorods are investigated in detail with focus on the collective effect due to lattice resonance (LR). Using an analytical approach based on the coupled dipole method (supported by full wave simulation), we find optical chirality is dramatically increased by the coupling between localized surface plasmon resonances and LR. The collective effect results in significant chiral signal even for metasurfaces made of achiral unit cells. The interlayer coupling generally destroys the Wood’s anomaly and the associated transparency. While making use of Pancharatnam–Berry (PB) phase and propagation phase, one can modulate the optical activity effectively and achieve chirality-selective transparency induced by LR in a designed structure with a g-factor of absorption as high as 1.99 (close to the upper limit of 2). Our studies not only reveal a new mechanism of modulating chiral optical response by combination effects from PB phase, propagation phase, and LR, but also give a quantitative relationship between the geometry configuration and chiral optical properties, thus providing helpful guidance for device design.

In the present study, an optical fiber surface plasmon resonance (SPR) biosensor was developed for measuring time- and concentration-dependent DNA hybridization kinetics. Its design complies with a 3D Au/Al2O3 multilayer composite hyperbolic metamaterial (HMM), a graphene film, and a D-shaped plastic optical fiber. According to the numerical simulation and the experimental demonstration, the SPR peak of the designed biosensor can be effectively altered in the range of visible to near-infrared by varying the HMM structure. The sensitivity of the appliance was shown to achieve a value of up to 4461 nm/RIU, allowing its applicability for bulk refractive index sensing. Furthermore, a biosensor designed in this work displayed high-resolution capability (ranging from 10 pM to 100 nM), good linearity, and high repeatability along with a detection limit down to 10 pM, thus suggesting a vast potential for medical diagnostics and clinical applications.

Recent advances of space-time-coding digital metasurfaces demonstrate powerful capabilities in the generation of nonlinear harmonics and the accurate control of the corresponding wavefronts. However, to date the near field manipulation and the experiment characterization are still not explored. In this paper, we propose a space-time-digital coding metasurface to realize accurate manipulation of the near fields at the fundamental and +1st (-1st) harmonics simultaneously, by properly controlling the initial phase and time delay of the time varying reflectivity. A novel mapping system is established to measure the nonlinear near field distributions of multiharmonics. Both the simulation and experimental results demonstrate the validity of the proposed method.

Characterizing the amplitude, phase profile, and polarization of optical beams is critical in modern optics. With a series of cascaded optical components, one can accurately resolve the optical singularity and polarization state in traditional polarimetry systems. However, complicated optical setups and bulky configurations inevitably hinder future applications for integration. Here, we demonstrate a metadevice that fully resolves arbitrary beams on a higher-order Poincaré sphere (HOPS) via a single-layer all-silicon metasurface. The device is compact and capable of detecting optical singularities and higher-order Stokes parameters simultaneously through a single intensity measurement. To verify the validity of the proposed metadevice, different beams on HOPS0,0 and HOPS1,-1 are illuminated on the metadevices. The beams are fully resolved, and the reconstructed higher-order Stokes parameters show good agreement with the original ones. Taking the signal-to-noise ratio into account, the numerical simulations indicate that the design strategy can be extended to fully resolve arbitrary beams on HOPS with order up to 4. Because of the advantages of compact configuration and compatibility with current semiconductor technology, the metadevice will facilitate potential applications in information processing and optical communications.

Depth of focus (DOF) and transverse resolution define the longitudinal range and definition of the focusing lens. Although metasurface axilenses and light-sword metalenses with radial and angular modulations can elongate the DOF, these approaches have inherent limitations in being reliable only for small numerical aperture (NA) cases, which in turn compromises the transverse resolution for the given aperture dimension. To conquer this limitation, we propose and experimentally demonstrate a birefringent metalens, achieving an ultradeep DOF of 41λ in terms of the total scattered field, corresponding to a record-breaking wide NA range from 0.14 to 0.7. Meanwhile, the diffraction limited focal spot size in this NA range can guarantee acquisition of images with high resolution. A hybrid methodology is proposed that utilizes both the accuracy of holography in electromagnetic field reconstruction and the polarization multiplexing to double the DOF. A stratified transmissive meta-atom is utilized to encode a pair of independent phase profiles in two orthogonal polarization channels. Furthermore, we combine the generalized scattering matrix with the multipole expansion theory for the first time to elucidate the mechanism of maintaining high transmittance and widening the transmission phase coverage by using the multilayered structure. The proposed metalens provides a competitive platform for devising high-resolution deep DOF systems for imaging and detection applications.

The direct interfacing of photonic crystal fiber to a metallic nanoantenna has widespread application in nanoscale imaging, optical lithography, nanoscale lasers, quantum communication, in vivo sensing, and medical surgery. We report on the fabrication of a needle-shaped plasmonic nanoantenna on the end facet of a photonic crystal fiber using electron-beam-induced evaporation of platinum. We demonstrate the coupling of light from the fiber waveguide mode to the subwavelength nanoantenna plasmonic mode focusing down to the apex of the plasmonic needle using a polarization-resolved far-field side-scatter imaging technique. Our work provides an important step toward widespread application of optical fibers in nearfield spectroscopic techniques such as tip-enhanced Raman and fluorescence microscopy, single-photon excitation and quantum sensors, nanoscale optical lithography, and lab-on-fiber devices.

Highly customized and miniaturized structured light is expected in many application fields. A kind of structured vortex generators is proposed based on a metasurface consisting of rectangular nanoholes etched in a silver film, and the generated vortices with the same or different topological charges are distributed along the radial direction. The geometric metasurface is completed with the help of optical holography technology, and the structured vortex generator possesses high working efficiency and large information capacity. The proposed vortex generators work under circularly polarized light illumination, and the reproduced vortices of multiplexing vortex generator depend on the handedness of the circularly polarized light. This work paves a way to generate new structured light fields. The radially distributed vortices may be utilized to simultaneously screen or separate microparticles. The compact design of the structured vortex generator and the convenient switch of different structured vortices will be a benefit to expand the applications of structured vortex fields.

Understanding the mode’s origin in planar metamaterials is fundamental for related applications in nanophotonics and plasmonics. For complex planar metamaterials, conventional analysis that directly obtains the final charge/current distribution of a mode is usually difficult in helping to understand the mode’s origin. In this paper, we propose a mode evolution method (MEM) with a core analysis tool, i.e., plasmonic evolution maps (PEMs), to describe the mode evolution in several complementary planar metamaterials with designed plasmonic atoms/molecules. The PEMs could not only clearly explain a mode’s origin, but also reveal the role of a structure’s symmetry in the mode formation process. The MEM with PEMs can work as a simple, efficient, and universal approach for the mode analysis in different kinds of planar metamaterials.

Mid-infrared thermal detectors have very important applications in the aerospace and military fields. However, due to the low heat transfer efficiency and slow response time, their application has been greatly restricted. Here, we theoretically demonstrate a dual-band perfect absorber for a mid-infrared detector based on a dielectric metal metasurface, and the optical and thermal properties are analyzed in detail. Simulation results show that the two narrow absorption peaks, corresponding to the absorption value of 97.5% at λ=6.142 μm with λFWHM≈40 nm and 99.7% at λ=7.795 μm with λFWHM≈80 nm, respectively, are achieved, and their different dependences on the structural parameters have been studied. A thermal detector at room temperature with total response time within 1.3 ms for dual-band and 0.4 ms for single-band is realized when the incident light flux is 1.0 W/cm2 for an average temperature increase of ΔT≈1.0 K. Our study offers a promising approach for designing a narrowband mid-infrared perfect absorber and a high-performance photodetector in nano-integrated photonics.

We have fabricated low-temperature grown GaAs (LT-GaAs)-based plasmonic photoconductive antennas by RF sputtering of Au nanoparticles and have evaluated their terahertz detection properties. Localized surface plasmon resonance enhances the electric fields near the surface and increases the optical absorption of nanoparticles. The resonance frequency depends on the density of electrons, the effective electron mass, and the size and shape of the nanoparticles. Therefore, we tried to develop a high-sensitivity LT-GaAs photoconductive detector (PCD), which is effective over a wide range of wavelengths, by RF sputtering of Au nano-islands with a variety of aspect ratios from 1.2 to 5.1 on the dipole gap region of the PCD. As a result, we succeeded in increasing the sensitivity by 29% and 40% in the amplitude of observed terahertz pulse for 800 nm and 1560 nm femtosecond laser excitations, respectively.

Dynamic control of compact chip-scale contactless manipulation of particles for bioscience applications remains a challenging endeavor, which is restrained by the balance between trapping efficiency and scalable apparatus. Metasurfaces offer the implementation of feasible optical tweezers on a planar platform for shaping the exerted optical force by a microscale-integrated device. Here we design and experimentally demonstrate a highly efficient silicon-based metalens for two-dimensional optical trapping in the near-infrared. Our metalens concept is based on the Pancharatnam–Berry phase, which enables the device for polarization-sensitive particle manipulation. Our optical trapping setup is capable of adjusting the position of both the metasurface lens and the particle chamber freely in three directions, which offers great freedom for optical trap adjustment and alignment. Two-dimensional (2D) particle manipulation is done with a relatively low-numerical-aperture metalens (NAML=0.6). We experimentally demonstrate both 2D polarization-sensitive drag and drop manipulation of polystyrene particles suspended in water and transfer of angular orbital momentum to these particles with a single tailored beam. Our work may open new possibilities for lab-on-a-chip optical trapping for bioscience applications and microscale to nanoscale optical tweezers.

Coupling effects of surface plasmon resonance (SPR) induce changes in the wavelength, intensity, and linewidth of plasmonic modes. Here, inspired by coupling effects, we reveal an abrupt linewidth-shrinking effect in 2D gold nanohole arrays at the azimuthal angle of 45° arising from the interference of two degenerate SPR modes. We further demonstrate the biosensing capability under various excitation conditions for detecting the critical molecular biomarker of prostatic carcinoma, and achieve the maximum sensitivity at this angle. Our study not only enhances the understanding toward plasmonic resonance-linewidth shrinking, but also provides a promising strategy to greatly improve biosensing performance by light manipulation on plasmonic nanostructures.

The field of chiral plasmonics has registered considerable progress with machine-learning (ML)-mediated metamaterial prototyping, drawing from the success of ML frameworks in other applications such as pattern and image recognition. Here, we present an end-to-end functional bidirectional deep-learning (DL) model for three-dimensional chiral metamaterial design and optimization. This ML model utilizes multitask joint learning features to recognize, generalize, and explore in detail the nontrivial relationship between the metamaterials’ geometry and their chiroptical response, eliminating the need for auxiliary networks or equivalent approaches to stabilize the physically relevant output. Our model efficiently realizes both forward and inverse retrieval tasks with great precision, offering a promising tool for iterative computational design tasks in complex physical systems. Finally, we explore the behavior of a sample ML-optimized structure in a practical application, assisting the sensing of biomolecular enantiomers. Other potential applications of our metastructure include photodetectors, polarization-resolved imaging, and circular dichroism (CD) spectroscopy, with our ML framework being applicable to a wider range of physical problems.

A low-loss hybrid plasmonic transverse magnetic (TM)-pass polarizer has been demonstrated utilizing polarization-dependent mode conversion. Taking advantage of the silicon hybrid plasmonic slot waveguide (HPSW), the unwanted transverse electric (TE) fundamental mode can be efficiently converted first to a TM higher-order mode and then suppressed by a power combiner, while the retained TM fundamental mode can pass through with negligible influence. Since the HPSW feature both strong structural asymmetry and a small interaction area in the cross-section between the metal and optical field, the optimized insertion loss of the device is as low as 0.4 dB. At the wavelength of 1550 nm, the extinction ratio is 28.3 dB with a moderate footprint of 2.38 μm×10 μm. For the entire C band, the average reflection of the TE mode is suppressed below ?14 dB, and the extinction ratio is over 18.6 dB. This work provides another more efficient and effective approach for better on-chip polarizers.

Tunable/reconfigurable metasurfaces that can actively control electromagnetic waves upon external stimuli are of great importance for practical applications of metasurfaces. Here, we demonstrate a reconfigurable nano-kirigami metasurface driven by pneumatic pressure operating in the near-infrared wavelength region. The metasurfaces consist of combined Archimedean spirals and are fabricated in a free-standing gold/silicon nitride nanofilm by employing focused ion beam (FIB) lithography. The deformable spirals are instantly transformed from two dimensional (2D) to three-dimensional (3D) by the FIB-based nano-kirigami process. The 2D–to–3D transformation induces a dramatic irreversible change of the plasmonic quadruple modes and results in significant modulation in reflection by 137%. The suspended porous nano-kirigami metasurface is further integrated with an optofluidics device, with which the optical resonance is reversibly modulated by the pneumatic pressure. This work provides a strategy for tunable/reconfigurable metasurfaces, which are useful to build a promising lab-on-a-chip platform for microfluidics, biological diagnostics, chemical sensing, and pressure monitoring.

Airy optical beams have emerged to hold enormous theoretical and experimental research interest due to their outstanding characteristics. Conventional approaches suffer from bulky and costly systems, as well as poor phase discretization. The newly developed metasurface-based Airy beam generators have constraints of polarization dependence or limited generation efficiency. Here, we experimentally demonstrate a polarization-independent silicon dielectric metasurface for generation of high-efficiency Airy optical beams. In our implementation, rather than synchronous manipulation of the amplitude and phase by plasmonic or Huygens’ metasurfaces, we employ and impose a 3/2 phase-only manipulation to the dielectric metasurface, consisting of an array of silicon nanopillars with an optimized transmission efficiency as high as 97%. The resultant Airy optical beams possess extraordinarily large deflection angles and relatively narrow beam widths. Our validated scheme will open up a fascinating doorway to broaden the application scenarios of Airy optical beams on ultracompact photonic platforms.

The comprehensive capture of near-field spatiotemporal information of surface plasmon polaritons (SPPs) is a prerequisite for revealing their physical nature. In this study, we first performed an independent, spatiotemporal imaging of the out-of-plane and in-plane components of SPP near-fields in a femtosecond light-excited trench using an obliquely incident time-resolved photoemission electron microscopy (TR-PEEM). We did the capture by imaging of the interference patterns induced by a superposition of the p- or s-polarized probe light, with the out-plane or in-plane components of SPP near-fields, under the noncollinear excitation mode. The method may be used to reconstruct a 3D SPP spatiotemporal field. Moreover, we demonstrated that the fringe shift of the interference patterns between the captured in-plane and out-of-plane components of the SPP field in PEEM images corresponds to the 1/4 fringe period, which is attributed to π/2 out of phase of the out-of-plane and in-plane near-field components of SPP. The resulting TR-PEEM images are supported by a classical wave mode and FDTD simulations. Essentially, the measured π/2 phase difference between the in-plane and out-of-plane components of the SPP indicated a rotating field component in the propagation plane, i.e., that the SPP exhibits an elliptically polarized electric field in the propagation plane. The experimental results presented herein provide direct evidence of SPP having the inherent attributes of transverse spin angular momentum.

With the recent development of the metasurface, generating an optical vortex in optical far or near fields is realized in various ways. However, to generate vortices in both the near and far fields simultaneously is still a challenge, which has great potential in the future compact and versatile photonic system. Here, a bi-channel optical vortex generator in both the near and far fields is proposed and demonstrated within a single metasurface, where the surface plasmon vortex and the far-field optical vortex can be simultaneously generated under circularly polarized light. The ability of generating vortices with arbitrary topological charges is experimentally demonstrated, which agrees well with simulations. This approach provides great freedom to integrate different vortex generators in a single device, and offers new opportunities for integrated optical communications, trapping, and other related fields.

Asymmetric transmission, defined as the difference between the forward and backward transmission, enables a plethora of applications for on-chip integration and telecommunications. However, the traditional method for asymmetric transmission is to control the propagation direction of the waves, hindering further applications. Metasurfaces, a kind of two-dimensional metamaterials, have shown an unprecedented ability to manipulate the propagation direction, phase, and polarization of electromagnetic waves. Here we propose and experimentally demonstrate a metasurface-based directional device consisting of a geometric metasurface with spatially rotated microrods and metallic gratings, which can simultaneously control the phase, polarization, and propagation direction of waves, resulting in asymmetric focusing in the terahertz region. These dual-layered metasurfaces for asymmetric focusing can work in a wide bandwidth ranging from 0.6 to 1.1 THz. The flexible and robust approach for designing broadband asymmetric focusing may open a new avenue for compact devices with potential applications in encryption, information processing, and communication.

The unwanted zero-order light accompanied by the birth of diffractive optical elements and caused mainly by fabrication errors and wavelength variations is a key factor that deteriorates the performance of diffraction-related optical devices such as holograms, gratings, beam shapers, beam splitters, optical diffusers, and diffractive microlenses. Here, inspired by the unique characteristic of nano-polarizer-based metasurfaces for both positive and negative amplitude modulation of incident light, we propose a general design paradigm to eliminate zero-order diffraction without burdening the metasurface design and fabrication. The experimentally demonstrated meta-hologram, which projects a holographic image with a wide angle of 70°×70° in the far field, presents a very low zero-order intensity (only 0.7% of the total energy of the reconstructed image). More importantly, the zero-order-free meta-hologram has a large tolerance limit for wavelength variations (under a broadband illumination from 520 to 660 nm), which brings important technical advances. The strategy proposed could significantly relieve the fabrication difficulty of metasurfaces and be viable for various diffractive-optics-related applications including holography, laser beam shaping, optical data storage, vortex beam generation, and so on.

Gap-surface plasmon (GSP) metasurfaces have attracted progressively increasing attention due to their planar configurations, ease of fabrication, and unprecedented capabilities in manipulating the reflected fields that enable integrating diverse bulk-optic-based optical components into a single ultrathin flat element. In this work, we design and experimentally demonstrate multifunctional metalenses that perform simultaneous linear-polarization conversion, focusing, and beam splitting, thereby reproducing the combined functionalities of conventional half-wave plates, parabolic reflectors, and beam splitters. The fabricated single-focal metalens incorporates properly configured distinct half-wave-plate-like GSP meta-atoms and exhibits good performance under linearly polarized incidence in terms of orthogonal linear-polarization conversion (>75%) and focusing (overall efficiency>22%) in the wavelength spectrum ranging from 800 to 950 nm. To further extend the combined functionalities, we demonstrate a dual-focal metalens that splits and focuses a linearly polarized incident beam into two focal spots while maintaining the capability of orthogonal linear-polarization conversion. Furthermore, the power distribution between two split beams can readily be controlled by judiciously positioning the incident beam. The demonstrated multifunctional GSP-based metalenses mimic the combined functionalities of a sequence of discrete bulk optical components, thereby eliminating the need for their mutual alignment and opening new perspectives in the development of ultracompact and integrated photonic devices.

Localized surface plasmon resonance (LSPR) of nanostructures and the interfacial charge transfer (CT) of semiconductor materials play essential roles in the study of optical and photoelectronic properties. In this paper, a composite substrate of Ag2S quantum dots (QDs) coated plasmonic Au bowtie nanoantenna (BNA) arrays with a metal–insulator–metal (MIM) configuration was built to study the synergistic effect of LSPR and interfacial CT using surface-enhanced Raman scattering (SERS) in the near-infrared (NIR) region. The Au BNA array structure with a large enhancement of the localized electric field (E-field) strongly enhanced the Raman signal of adsorbed p-aminothiophenol (PATP) probe molecules. Meanwhile, the broad enhanced spectral region was achieved owing to the coupling of LSPR. The as-prepared Au BNA array structure facilitated enhancements of the excitation as well as the emission of Raman signal simultaneously, which was established by finite-difference time-domain simulation. Moreover, Ag2S semiconductor QDs were introduced into the BNA/PATP system to further enhance Raman signals, which benefited from the interfacial CT resonance in the BNA/Ag2S-QDs/PATP system. As a result, the Raman signals of PATP in the BNA/Ag2S-QDs/PATP system were strongly enhanced under 785 nm laser excitation due to the synergistic effect of E-field enhancement and interfacial CT. Furthermore, the SERS polarization dependence effects of the BNA/Ag2S-QDs/PATP system were also investigated. The SERS spectra indicated that the polarization dependence of the substrate increased with decreasing polarization angles (θpola) of excitation from p-polarized (θpola=90°) excitation to s-polarized (θpola=0°) excitation. This study provides a strategy using the synergistic effect of interfacial CT and E-field enhancement for SERS applications and provides a guidance for the development of SERS study on semiconductor QD-based plasmonic substrates, and can be further extended to other material-nanostructure systems for various optoelectronic and sensing applications.

The real-time measurement of the polarization and phase information of light is very important and desirable in optics. Metasurfaces can be used to achieve flexible wavefront control and can therefore be used to replace traditional optical elements to produce a highly integrated and extremely compact optical system. Here, we propose an efficient and compact optical multiparameter detection system based on a Hartmann–Shack array with 2×2 subarray metalenses. This system not only enables the efficient and accurate measurement of the spatial polarization profiles of optical beams via the inspection of foci amplitudes, but also measures the phase and phase-gradient profiles by analyzing foci displacements. In this work, details of the design of the elliptical silicon pillars for the metalens are described, and we achieve a high average focusing efficiency of 48% and a high spatial resolution. The performance of the system is validated by the experimental measurement of 22 scalar polarized beams, an azimuthally polarized beam, a radially polarized beam, and a vortex beam. The experimental results are in good agreement with theoretical predictions.

Metamaterials play an important role in the modulation of amplitude and group delay in the terahertz (THz) regime on account of their optical properties, which are rare in natural materials. Here an ultrafast anisotropic switch of the plasmon-induced transparency (PIT) effect is experimentally and numerically demonstrated by metamaterial devices composed of two pairs of planar split-ring resonators and a pair of closed-ring resonators. By integration with a germanium (Ge) film, a recovery time of 3 ps and a decay constant of 785 fs are realized in the metadevice. Stimulated by the exterior optical pump, the PIT windows at different frequencies are switched off with an excellent property of slow light for vertical and horizontal THz polarizations, realizing an astonishing modulation depth as high as 99.06%. This work provides a new platform for ultrafast anisotropic metadevices tunable for amplitude and group delay.

Gap-type metallic nanostructures are widely used in catalytic reactions, sensors, and photonics because the hotspot effect on these nanostructures supports giant local electromagnetic field enhancement. To achieve hotspots, researchers devote themselves to reducing gap distances, even to 1 nm. However, current techniques to fabricate such narrow gaps in large areas are still challenging. Herein, a new coupling way to boost the sub-10 nm plasmonic nanogap array is developed, based on the plasmon-triggered optical waveguide resonance via near-field coupling. This effect leads to an amplified local electromagnetic field within the gap regions equivalent to narrower gaps, which is evidenced experimentally by the surface-enhanced Raman scattering intensity of probed molecules located in the gap and the finite-difference time-domain numerical simulation results. This study provides a universal strategy to promote the performance of the existing hotspot configurations without changing their geometries.

Magneto-plasmonic sensors based on surface plasmon resonance have been studied considerably in recent years, as they feature high sensitivity and ultrahigh resolution. However, the majority of such investigations focus on prism-based sandwich architectures that not only impede the miniaturization of devices but also have a weak transverse magneto-optical Kerr effect (TMOKE) in magnitude. Herein, we theoretically demonstrate a magneto-plasmonic sensor composed of Au/Co bilayer nanodisk arrays on top of optically thick metallic films, which supports a narrow surface plasmon resonance (SPR) with a bandwidth of 7 nm and allows for refractive index sensitivities as high as 717 nm/RIU. Thanks to the high-quality SPR mode, a Fano-like TMOKE spectrum with a subnanometer bandwidth can be achieved in the proposed structure, thereby giving rise to ultrahigh sensing of merit values as large as 7000 in water. Moreover, we demonstrate a large TMOKE magnitude that exceeds 0.6. The value is 1 order of magnitude larger than that of magneto-plasmonic sensors reported. We also demonstrate that the behavior of TMOKE spectra can be controlled by tuning the geometrical parameters of the device including the diameter and thickness of nanodisk arrays. This work provides a promising route for designing magneto-plasmonic sensors based on metasurfaces or metamaterials.

Tip-enhanced Raman spectroscopy (TERS) offers a powerful means to enhance the Raman scattering signal of a molecule as the localized surface plasmonic resonance will induce a significant local electric field enhancement in the nanoscale hot spot located within the nanogap of the TERS system. In this work, we theoretically show that this nanoscale hot spot can also serve as powerful optical tweezers to tightly trap a molecule. We calculate and analyze the local electric field and field gradient distribution of this nanogap plasmon hot spot. Due to the highly localized electric field, a three-dimensional optical trap can form at the hot spot. Moreover, the optical energy density and optical force acting on a molecule can be greatly enhanced to a level far exceeding the conventional single laser beam optical tweezers. Calculations show that for a single H2TBPP organic molecule, which is modeled as a spherical molecule with a radius of rm=1 nm, a dielectric coefficient ε=3, and a polarizability α=4.5×10-38 C·m2/V, the stiffness of the hot-spot trap can reach a high value of about 2 pN/[(W/cm2)·m] and 40 pN/[(W/cm2)·m] in the direction perpendicular and parallel to the TERS tip axis, which is far larger than the stiffness of single-beam tweezers, ～0.4 pN/[(W/cm2)·m]. This hard-stiffness will enable the molecules to be stably captured in the plasmon hot spot. Our results indicate that TERS can become a promising tool of optical tweezers for trapping a microscopic object like molecules while implementing Raman spectroscopic imaging and analysis at the same time.

Flat optics presents a new path to control the phase, amplitude, and polarization state of light with ultracompact devices. Here we demonstrate chip-integrated metasurface devices for polarization detection of mid-infrared light with arbitrary polarization states. Six high-performance microscale linear and circular polarization filters based on vertically stacked plasmonic metasurfaces (with total thickness <600 nm) are integrated on the same chip to obtain all four Stokes parameters of light with high accuracy. The device designs can be tailored to operate at any wavelength in the mid-infrared spectral region and are feasible for on-chip integration with mid-infrared (mid-IR) photodetectors and imager arrays. Our work will enable on-chip mid-IR polarimeters and polarimetric imaging systems, which are highly desirable for many applications, such as clinic diagnosis, target detection, and space exploration.

Optical absorbers with dynamic tuning features are able to flexibly control the absorption performance, which offers a good platform for realizing optical switching, filtering, modulating, etc. Here, we propose a thermally tunable broadband absorber applying a patterned plasmonic metasurface with thermo-chromic vanadium dioxide (VO2) spacers. An actively tunable absorption bandwidth and peak resonant wavelength in the region from the near- to mid-infrared (NMIR) are simultaneously achieved with the insulating–metallic phase transition of VO2. Moreover, the scalable unit cell, which is composed of multi-width sub-cells, provides a new freedom to further manipulate (i.e., broaden or narrow) the absorption bandwidth while maintaining a high relative absorption bandwidth and efficient absorbance at the same time. For both transverse-electric and transverse-magnetic polarizations, the proposed nanostructure exhibits a high absorption over a wide angular range up to 60°. This method holds a promising potential for versatile utilizations in optical integrated devices, NMIR photodetection, thermal emitters, smart temperature control systems, and so forth.

In this study, a point-scattering approach to the plane-wave optical transmission of subwavelength metal nanoslit arrays with varying angles of rotation and that of subwavelength metal supercell arrays consisting of nanoslits capable of various angles of rotation is developed. It is demonstrated that the suggested theories show good agreement with the simulations and experiments. The results show that constructive and destructive interference at each nanoslit can respectively enhance and suppress the surface plasmon polariton (SPP) far-field radiation of a metasurface. The proposed theory can predict the quantity and resonant wavelength of SPPs and provide a design scheme for an SPP device.

We experimentally demonstrate a scheme to deterministically excite a three-dimensionally oriented electric dipole in a single Au nanosphere by using a tightly focused radially polarized beam whose focal field possesses polarization states along three-dimensional (3D) orientations owing to the spatial overlap between longitudinal and radial electric field components. Experiment observations indicate that the orientation of an excited dipole moment gradually changes from out-of-plane to in-plane when the nanosphere is moved away from the beam center, which is reconfirmed by full-wave simulations. Moreover, rigorous calculation based on Mie theory reveals that a reduced effective ambient permittivity accompanies the rotation of the dipole moment, leading to a blue-shifted and narrowed resonance peak. We envision that our results could find applications in detecting the 3D orientation of isolated molecules and benefit the fine manipulation of light–matter interactions at the single-molecule level.

In this work, we present a multi-channel nonreciprocal waveguide, which is composed of a gyrotropic-bounded dielectric on the bottom and a plasmonic material on the top. The Lorentz reciprocity in the time-invariant system is broken when applying an external static magnetic field on the gyrotropic material. The nonreciprocal emission from the dipole source located in the center of the waveguide is observed in extended waveband channels. The proposed heterostructure serves as a photonic dichroism once the dielectric is replaced by a nonlinear material. The associated second harmonic generated in the nonlinear process can be separated from the fundamental signal under proper magnetic field intensity. Our findings may provide significant guidance for designing nonreciprocal photonic devices with superiorities of a tunable waveband, multiple channels, and small footprint.

Bio-chemical molecular detection in the nanoscale, based on alloyed nanorods (NRs) with tunable surface plasmon resonance (SPR) properties and high chemical stability, has attracted particular interest. In this work, alloyed Au-Ag NRs with tunable aspect ratios were achieved by annealing Au nanobipyramid-directed Au@Ag core-shell NRs. The core-shell NRs were encapsulated within mesoporous silica outer shells to avoid fusion or aggregation. The structural stability of fully alloyed Au-Ag NRs, including chemical and thermal stability, is remarkably improved compared with that of Au@Ag core-shell NRs. The alloyed NRs would maintain the rod-like structure after being incubated in etchant solution, while Au@Ag core-shell NRs would decay into nanobipyramids. Additionally, fully alloyed NRs present stable morphology under annealing at high temperatures of up to 600°C in air. Benefiting from excellent structural and chemical stabilities, the surface-enhanced Raman scattering effect based on alloyed NRs is stable in harsh environments. Taking advantage of tunable SPR properties (600–1800 nm) and excellent stability, the obtained nanostructures can serve as drug carriers. The perfect photo-thermal effect induced by the particular SPR of alloyed NRs can improve the release efficiency of drugs.

The synergy of a plasmonic tip and fiber-based structure light field excitation can provide a powerful tool for Raman examination. Here, we present a method of Raman spectrum enhancement with an Ag-nanoparticles (Ag-NPs)-coated fiber probe internally excited via an azimuthal vector beam (AVB), which is directly generated in a few-mode fiber by using an acoustically induced fiber grating. Theoretical analysis shows that gap mode can be effectively generated on the surface of the Ag-NPs-coated fiber probe excited via an AVB. The experimental result shows that the intensity of Raman signal obtained with analyte molecules of malachite green by exciting the Ag-NPs-coated fiber probe via an AVB is approximately eight times as strong as that via the linear polarization beam (LPB), and the activity of the AVB-excited fiber probe can reach 10 11 mol/L, which cannot be achieved by LPB excitation. Moreover, the time stability and reliability are also examined, respectively.

Because they possess excellent visible light absorption properties, lead-free colloidal copper-based chalcogenide quantum dots (QDs) have emerged in photoelectronic fields. By means of localized surface plasmonic resonance (LSPR), the absorption properties of QDs can be enhanced. In this paper, we fabricate a lead-free CuInSe2 QD field effect phototransistor (FEpT) by utilizing the LSPR enhancement of Au nanoparticles (NPs). The plasmonic FEpT demonstrates responsivity up to 2.7 μA·W 1 and a specific detectivity of 7×103 Jones at zero bias under illumination by a 532 nm laser, values that are enhanced by approximately 200% more than devices without Au NPs. Particularly, the FEpT exhibits a multi-wavelength response, which is photoresponsive to 405, 532, and 808 nm irradiations, and presents stability and reproducibility in the progress of ON–OFF cycles. Furthermore, the enhancement induced by Au NP LSPR can be interpreted by finite-difference time domain simulations. The low-cost solution-based process and excellent device performance strongly underscore lead-free CuInSe2 QDs as a promising material for self-powered photoelectronic applications, which can be further enhanced by Au NP LSPR.

Metasurfaces have pioneered a new avenue for advanced wave-front engineering. Among the various types of metasurfaces, Huygens’ metasurfaces are thought to be a novel paradigm for flat optical devices. Enabled by spectrally overlapped electric resonance and magnetic resonance, Huygens’ metasurfaces are imparted with high transmission and full phase coverage of 2π, which makes them capable of realizing high-efficiency wave-front control. However, a defect of Huygens’ metasurfaces is that their phase profiles and transmissive responses are often sensitive to the interaction of neighboring Huygens’ elements. Consequently, the original assigned phase distribution can be distorted. In this work, we present our design strategy of transmissive Huygens’ metasurfaces performing anomalous refraction. We illustrate the investigation of Huygens’ elements, realizing the overlapping between an electric dipole and magnetic dipole resonance based on cross-shaped structures. We find that the traditional discrete equidistant-phase design method is not enough to realize a transmissive Huygens’ surface due to the interaction between neighboring Huygens’ elements. Therefore, we introduce an extra optimization process on the element spacing to palliate the phase distortion resulting from the element interaction. Based on this method, we successfully design unequally spaced three-element transmissive metasurfaces exhibiting anomalous refraction effect. The anomalous refractive angle of the designed Huygens’ metasurface is 30°, which exceeds the angles of most present transmissive Huygens’ metasurfaces. A transmissive efficiency of 83.5% is numerically derived at the operating wavelength. The far-field electric distribution shows that about 93% of transmissive light is directed along the 30° refractive direction. The deflection angle can be tuned by adjusting the number of Huygens’ elements in one metasurface unit cell. The design strategies used in this paper can be inspiring for other functional Huygens’ metasurface schemes.

Surface-enhanced Raman spectroscopy (SERS) with high-sensitivity performance is a very necessary detection technology. Here, we present a method for increasing the performance of SERS based on silver triangular nanoprism arrays (ATNAs) vertically excited via a focused azimuthal vector beam (AVB). The ATNA substrates with different structural parameters are prepared based on the traditional self-assembled and modified film lift-off technique. Based on a theoretical model established adopting the structural parameters of the ATNA substrates, theoretical simulation results show that AVB excitation can achieve greater electric-field enhancement than linearly polarized beam (LPB) excitation. Experimental result indicates that SERS sensitivity obtained via AVB excitation is 10 13 M (1 M = 1 mol/L) using rhodamine 6G (R6G) as the target analyte, which is 2 orders of magnitude lower than that of LPB excitation (10 11 M). Meanwhile, the uniformity and reproducibility of the ATNA substrates are examined using Raman mapping and batch-to-batch measurement, respectively, and the Raman enhancement factor is calculated to be ～3.3×107. This method of vector light field excitation may be used to improve the SERS performance of the substrates in fields of ultra-sensitive Raman detection.

A depletion layer played by aqueous organic liquids flowing in a platform of microfluidic integrated metamaterials is experimentally used to actively modulate terahertz (THz) waves. The polar configuration of water molecules in a depletion layer gives rise to a damping of THz waves. The parallel coupling of the damping effect induced by a depletion layer with the resonant response by metamaterials leads to an excellent modulation depth approaching 90% in intensity and a great difference over 210° in phase shift. Also, a tunability of slow-light effect is displayed. Joint time-frequency analysis performed by the continuous wavelet transforms reveals the consumed energy with varying water content, indicating a smaller moment of inertia related to a shortened relaxation time of the depletion layer. This work, as part of THz aqueous photonics, diametrically highlights the availability of water in THz devices, paving an alternative way of studying THz wave–liquid interactions and developing active THz photonics.

We present a new design of a plasmonic Luneburg lens made from a gradient-index metasurface that was constructed with an array of nanometer-sized holes in a dielectric thin film. The fabricated structure consists of a planar lens with a diameter of 8.7 μm composed of a rectangular array of holes with a periodicity of 300 nm. The experimental characterization includes leakage-radiation microscopy imaging in the direction and frequency space. The former allows for characterization of the point spread function and phase distribution, whereas the latter grants access to qualitative measurements of the effective mode indices inside the plasmonic lens. The experimental results presented here are in good agreement with the expected average performance predicted by the numerical calculations. Nevertheless, the robustness of the characterization techniques presented here is also exploited to determine deviations from the design parameters.

Polarization manipulation is a significant issue for artificial modulation of the electromagnetic (EM) wave, but general mechanisms all suffer the restriction of inherent symmetric properties between opposite handedness. Herein, a strategy to independently and arbitrarily manipulate the EM wave with orthogonal circular polarizations based on a metasurface is proposed, which effectually breaks through traditional symmetrical characteristics between orthogonal handedness. By synthesizing the propagation phase and geometric phase, the appropriate Jones matrix is calculated to obtain independent wavefront manipulation of EM waves with opposite circular polarizations. Two transmissive ultra-thin meta-deflectors are proposed to demonstrate the asymmetrical refraction of transmitted circularly polarized waves in the microwave region. Simulated transmitted phase front and measured far-field intensity distributions are in excellent agreement, indicating that the transmitted wave with different polarizations can be refracted into arbitrary and independent directions within a wide frequency band (relative bandwidth of 25%). The results presented in this paper provide more freedom for the manipulation of EM waves, and motivate the realizations of various polarization-independent properties for all frequency spectra.